Advances in reduction of NOx and N2O1 emission formation in an oxyfired fluidized bed boiler

doi:10.1016/j.cjche.2018.06.033

Chin.J.Chem.Eng. ›› 2019, Vol. 27 ›› Issue (2): 426-443.DOI: 10.1016/j.cjche.2018.06.033

• Energy, Resources and Environmental Technology • Previous Articles Next Articles

Advances in reduction of NO_x and N₂O1 emission formation in an oxyfired fluidized bed boiler

Khalid El Sheikh^1,2, Mohammad Jakir Hossain Khan², Mahar Diana Hamid², Siddhartha Shrestha³, Brahim Si Ali², G.A. Ryabov⁴, Lya A. Dolgushin⁴, Mohd Azlan Hussain², Tatiana V. Bukharkina¹, Elena A. Gorelova⁴

1 Dmitry Mendeleev University of Chemical Technology of Russia, Moscow 125047, Russia;
2 Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia;
3 Laboratory for Simulation and Modelling of Particulate Systems, Department of Chemical Engineering, Monash University, Victoria 3800, Australia.;
4 All-Russian Thermal Engineering Institute, VTI, 14/23 Avtozavodskaya str, Moscow, Russia

Received:2018-01-11 Revised:2018-06-10 Online:2019-03-18 Published:2019-02-28
Contact: Khalid El Sheikh, Mohammad Jakir Hossain Khan
Supported by:
Supported by the University of Malaya, Ministry of Education Malaysia under the grant FP064-2015A (FRGS) and IPPP grant number: PG101-2015B

Advances in reduction of NO_x and N₂O1 emission formation in an oxyfired fluidized bed boiler

1 Dmitry Mendeleev University of Chemical Technology of Russia, Moscow 125047, Russia;
2 Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia;
3 Laboratory for Simulation and Modelling of Particulate Systems, Department of Chemical Engineering, Monash University, Victoria 3800, Australia.;
4 All-Russian Thermal Engineering Institute, VTI, 14/23 Avtozavodskaya str, Moscow, Russia

通讯作者: Khalid El Sheikh, Mohammad Jakir Hossain Khan
基金资助:
Supported by the University of Malaya, Ministry of Education Malaysia under the grant FP064-2015A (FRGS) and IPPP grant number: PG101-2015B

Abstract

Abstract: Fossil fuel combustion is one of the major means to meet the mounting global energy demand. However, the increasing NO_x and N₂O emissions arising from fossil fuel combustion process have hazardous effects. Thus, mitigating these gases is vital to attain a sustainable environment. Interestingly, oxy-fuel combustion in fluidized bed for carbon capture and minimized NO_x emissions is strongly sustainable compare to the other approaches. It was assessed that NO_x formation and fuel-N conversion have significant limitation under oxy-fluidized bed compared to air mode and the mechanism of NO_x formation is still deficient and requires further development. In addition, this review paper discussed the potential of primary measure as low emission process with others supplementary techniques for feasible NO_x reduction. The influences of combustion mode, operating parameters, and reduction techniques such as flue gas recirculation, oxygen staging, biomass co-firing, catalyst, influence of fluidized bed design and structure, decoupling combustion and their merges are respectively evaluated. Findings show that significant minimization of NO_x emission can be achieved through combination of primary and secondary reduction techniques.

Key words: Oxy-fuel combustion, Fluidized bed technology, Biomass blend, Primary/ secondary measures, NO_x emission

摘要： Fossil fuel combustion is one of the major means to meet the mounting global energy demand. However, the increasing NO_x and N₂O emissions arising from fossil fuel combustion process have hazardous effects. Thus, mitigating these gases is vital to attain a sustainable environment. Interestingly, oxy-fuel combustion in fluidized bed for carbon capture and minimized NO_x emissions is strongly sustainable compare to the other approaches. It was assessed that NO_x formation and fuel-N conversion have significant limitation under oxy-fluidized bed compared to air mode and the mechanism of NO_x formation is still deficient and requires further development. In addition, this review paper discussed the potential of primary measure as low emission process with others supplementary techniques for feasible NO_x reduction. The influences of combustion mode, operating parameters, and reduction techniques such as flue gas recirculation, oxygen staging, biomass co-firing, catalyst, influence of fluidized bed design and structure, decoupling combustion and their merges are respectively evaluated. Findings show that significant minimization of NO_x emission can be achieved through combination of primary and secondary reduction techniques.

关键词: Oxy-fuel combustion, Fluidized bed technology, Biomass blend, Primary/ secondary measures, NO_x emission

Khalid El Sheikh, Mohammad Jakir Hossain Khan, Mahar Diana Hamid, Siddhartha Shrestha, Brahim Si Ali, G.A. Ryabov, Lya A. Dolgushin, Mohd Azlan Hussain, Tatiana V. Bukharkina, Elena A. Gorelova. Advances in reduction of NO_x and N₂O1 emission formation in an oxyfired fluidized bed boiler[J]. Chin.J.Chem.Eng., 2019, 27(2): 426-443.

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Advances in reduction of NO_x and N₂O1 emission formation in an oxyfired fluidized bed boiler

Advances in reduction of NO_x and N₂O1 emission formation in an oxyfired fluidized bed boiler

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