The latest development on amine functionalized solid adsorbents for post-combustion CO2 capture: Analysis review

doi:10.1016/j.cjche.2020.11.028

Chinese Journal of Chemical Engineering ›› 2021, Vol. 35 ›› Issue (7): 17-43.DOI: 10.1016/j.cjche.2020.11.028

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The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review

Peiyu Zhao^1,2, Guojie Zhang², Huangyu Yan², Yuqiong Zhao²

1. Heze Branch, Qilu University of Technology (Shandong Academy of Sciences), Biological Engineering Technology Innovation Center of Shandong Province, Heze 274000, China;
2. Key Laboratory of Coal Science and Technology, Ministry of Education and Shanxi Province, Taiyuan University of Technology, Taiyuan 030024, China

Received:2020-06-07 Revised:2020-10-06 Online:2021-09-30 Published:2021-07-28
Contact: Guojie Zhang
Supported by:
This work was supported by the National Natural Science Foundation of China (21878200 and 21676174), International S&T Cooperation Program of Shanxi province (201703D421038), Shanxi Scholarship Council of China (2017-036), and Joint Fund of Shanxi Provincial Coal Seam Gas (2015012019).

The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review

Peiyu Zhao^1,2, Guojie Zhang², Huangyu Yan², Yuqiong Zhao²

1. Heze Branch, Qilu University of Technology (Shandong Academy of Sciences), Biological Engineering Technology Innovation Center of Shandong Province, Heze 274000, China;
2. Key Laboratory of Coal Science and Technology, Ministry of Education and Shanxi Province, Taiyuan University of Technology, Taiyuan 030024, China

通讯作者: Guojie Zhang
基金资助:
This work was supported by the National Natural Science Foundation of China (21878200 and 21676174), International S&T Cooperation Program of Shanxi province (201703D421038), Shanxi Scholarship Council of China (2017-036), and Joint Fund of Shanxi Provincial Coal Seam Gas (2015012019).

Abstract

Abstract: Global warming and associated global climate change have led to serious efforts towards reducing CO₂ emissions through the CO₂ capture from the major emission sources. CO₂ capture using the amine functionalized adsorbents is regard as a direct and effective way to reducing CO₂ emissions due to their large CO₂ adsorption amount, excellent CO₂ adsorption selectivity and lower energy requirements for adsorbent regeneration. Moreover, large number of achievements on the amine functionalized solid adsorbent have been recorded for the enhanced CO₂ capture in the past few years. In view of this, we review and analyze the recent advances in amine functionalized solid adsorbents prepared with different supporting materials including mesoporous silica, zeolite, porous carbon materials, metal organic frameworks(MOF) and other composite porous materials. In addition, amine functionalized solid adsorbents derived from waste resources are also reviewed because of the large number demand for cost-effective carbon dioxide adsorbents and the processing needs of waste resources. Considering the importance of the stability of the adsorbent in practical applications, advanced research in the capture cycle stability has also been summarized and analyzed. Finally, we summarize the review and offer the recommendations for the development of amine-based solid adsorbents for carbon dioxide capture.

Key words: Solid adsorbents, Amine functionalized, CO₂ capture, Adsorption, Review

摘要： Global warming and associated global climate change have led to serious efforts towards reducing CO₂ emissions through the CO₂ capture from the major emission sources. CO₂ capture using the amine functionalized adsorbents is regard as a direct and effective way to reducing CO₂ emissions due to their large CO₂ adsorption amount, excellent CO₂ adsorption selectivity and lower energy requirements for adsorbent regeneration. Moreover, large number of achievements on the amine functionalized solid adsorbent have been recorded for the enhanced CO₂ capture in the past few years. In view of this, we review and analyze the recent advances in amine functionalized solid adsorbents prepared with different supporting materials including mesoporous silica, zeolite, porous carbon materials, metal organic frameworks(MOF) and other composite porous materials. In addition, amine functionalized solid adsorbents derived from waste resources are also reviewed because of the large number demand for cost-effective carbon dioxide adsorbents and the processing needs of waste resources. Considering the importance of the stability of the adsorbent in practical applications, advanced research in the capture cycle stability has also been summarized and analyzed. Finally, we summarize the review and offer the recommendations for the development of amine-based solid adsorbents for carbon dioxide capture.

关键词: Solid adsorbents, Amine functionalized, CO₂ capture, Adsorption, Review

Peiyu Zhao, Guojie Zhang, Huangyu Yan, Yuqiong Zhao. The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review[J]. Chinese Journal of Chemical Engineering, 2021, 35(7): 17-43.

Peiyu Zhao, Guojie Zhang, Huangyu Yan, Yuqiong Zhao. The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review[J]. 中国化学工程学报, 2021, 35(7): 17-43.

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The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review

The latest development on amine functionalized solid adsorbents for post-combustion CO₂ capture: Analysis review

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