Enhanced recycling performance of bimetallic Ir-Re/SiO2 catalyst by amberlyst-15 for glycerol hydrogenolysis

doi:10.1016/j.cjche.2021.07.015

Chinese Journal of Chemical Engineering ›› 2022, Vol. 45 ›› Issue (5): 171-181.DOI: 10.1016/j.cjche.2021.07.015

Previous Articles Next Articles

Enhanced recycling performance of bimetallic Ir-Re/SiO₂ catalyst by amberlyst-15 for glycerol hydrogenolysis

Xin Ren¹, Li Leng¹, Yueqiang Cao¹, Jing Zhang¹, Xuezhi Duan¹, Xueqing Gong², Jinghong Zhou¹, Xinggui Zhou¹

1 State Key Laboratory of Chemical Engineering, East China University of Science and Technology, Shanghai 200237, China;
2 Key Laboratory for Advanced Materials, Centre for Computational Chemistry and Research Institute of Industrial Catalysis, East China University of Science and Technology, Shanghai 200237, China

Received:2021-02-08 Revised:2021-06-26 Online:2022-06-22 Published:2022-05-28
Contact: Yueqiang Cao,E-mail:yqcao@ecust.edu.cn;Jinghong Zhou,E-mail:jhzhou@ecust.edu.cn
Supported by:
This work was supported by Ministry of Science and Technology of the People’s Republic of China, under the Research Fund for National Key R&D Program of China (2018YFB0604700), the Natural Science Foundation of China (22008067, 22008074, 22008072, 21991103), the China Postdoctoral Science Foundation (2020M681202 and 2021T140204) and Natural Science Foundation of Shanghai (20ZR1415700).

Enhanced recycling performance of bimetallic Ir-Re/SiO₂ catalyst by amberlyst-15 for glycerol hydrogenolysis

Xin Ren¹, Li Leng¹, Yueqiang Cao¹, Jing Zhang¹, Xuezhi Duan¹, Xueqing Gong², Jinghong Zhou¹, Xinggui Zhou¹

1 State Key Laboratory of Chemical Engineering, East China University of Science and Technology, Shanghai 200237, China;
2 Key Laboratory for Advanced Materials, Centre for Computational Chemistry and Research Institute of Industrial Catalysis, East China University of Science and Technology, Shanghai 200237, China

通讯作者: Yueqiang Cao,E-mail:yqcao@ecust.edu.cn;Jinghong Zhou,E-mail:jhzhou@ecust.edu.cn
基金资助:
This work was supported by Ministry of Science and Technology of the People’s Republic of China, under the Research Fund for National Key R&D Program of China (2018YFB0604700), the Natural Science Foundation of China (22008067, 22008074, 22008072, 21991103), the China Postdoctoral Science Foundation (2020M681202 and 2021T140204) and Natural Science Foundation of Shanghai (20ZR1415700).

Abstract

Abstract: Recycling performance of heterogeneous catalysts is of crucial importance especially for a batch reaction system. In this work, we demonstrate a strategy for enhancing recycling performance of Ir-Re/SiO₂ catalyst synergized with amberlyst-15 in glycerol hydrogenolysis to produce 1,3-propanediol. Comprehensive characterization results reveal that the Re sites in the Ir-Re/SiO₂ catalyst undergo irreversible segregation and oxidation. These hinder the formation of active Re—OH species and thus contribute to a complete and irreversible deactivation. However, the introduction of amberlyst-15 into the reactant mixture can restrain the oxidation process of Re sites and favor the formation of Re—OH species, and thus significantly enhance the catalytic recycling performance. The results demonstrated here could guide the development of excellent bimetallic catalysts with the desirable recycling performances for the reaction.

Key words: Glycerol hydrogenolysis, Ir-Re/SiO₂ catalyst, Deactivation mechanism, Recycling performance, Amberlyst-15 promoter

摘要： Recycling performance of heterogeneous catalysts is of crucial importance especially for a batch reaction system. In this work, we demonstrate a strategy for enhancing recycling performance of Ir-Re/SiO₂ catalyst synergized with amberlyst-15 in glycerol hydrogenolysis to produce 1,3-propanediol. Comprehensive characterization results reveal that the Re sites in the Ir-Re/SiO₂ catalyst undergo irreversible segregation and oxidation. These hinder the formation of active Re—OH species and thus contribute to a complete and irreversible deactivation. However, the introduction of amberlyst-15 into the reactant mixture can restrain the oxidation process of Re sites and favor the formation of Re—OH species, and thus significantly enhance the catalytic recycling performance. The results demonstrated here could guide the development of excellent bimetallic catalysts with the desirable recycling performances for the reaction.

关键词: Glycerol hydrogenolysis, Ir-Re/SiO₂ catalyst, Deactivation mechanism, Recycling performance, Amberlyst-15 promoter

Xin Ren, Li Leng, Yueqiang Cao, Jing Zhang, Xuezhi Duan, Xueqing Gong, Jinghong Zhou, Xinggui Zhou. Enhanced recycling performance of bimetallic Ir-Re/SiO₂ catalyst by amberlyst-15 for glycerol hydrogenolysis[J]. Chinese Journal of Chemical Engineering, 2022, 45(5): 171-181.

References

[1] K. Chen, M. Tamura, Z. Yuan, Y. Nakagawa, K. Tomishige, One-Pot Conversion of Sugar and Sugar Polyols to n-Alkanes without C-C Dissociation over the Ir-ReOx/SiO₂ Catalyst Combined with H-ZSM-5, ChemSusChem, 6 (2013) 613-621
[2] M. Gu, L. Liu, Y. Nakagawa, C. Li, M. Tamura, Z. Shen, X. Zhou, Y. Zhang, K. Tomishige, Selective Hydrogenolysis of Erythritol over Ir-ReOx/Rutile-TiO₂ Catalyst, ChemSusChem, 14 (2021) 489-489
[3] S. Liu, Y. Amada, M. Tamura, Y. Nakagawa, K. Tomishige, Performance and characterization of rhenium-modified Rh-Ir alloy catalyst for one-pot conversion of furfural into 1, 5-pentanediol, Catal. Sci. Technol., 4 (2014) 2535-2549
[4] S. Liu, Y. Okuyama, M. Tamura, Y. Nakagawa, A. Imai, K. Tomishige, Production of Renewable Heanols from Mechanocatalytically Depolymerized Cellulose by Using Ir-ReOx/SiO₂ catalyst, ChemSusChem, 8 (2015) 628-635
[5] S. Liu, Y. Okuyama, M. Tamura, Y. Nakagawa, A. Imai, K. Tomishige, Catalytic conversion of sorbitol to gasoline-ranged products without external hydrogen over Pt-modified Ir-ReOx/SiO₂, Catal. Today, 269 (2016) 122-131
[6] S. Liu, Y. Okuyama, M. Tamura, Y. Nakagawa, A. Imai, K. Tomishige, Selective transformation of hemicellulose (xylan) into n-pentane, pentanols or xylitol over a rhenium-modified iridium catalyst combined with acids, Green Chem., 18 (2016) 165-175
[7] S. Liu, M. Tamura, Y. Nakagawa, K. Tomishige, One-pot conversion of cellulose into n-hexane over the Ir-ReOx/SiO₂ catalyst combined with HZSM-5, ACS Sustainable Chem. Eng., 2 (2014) 1819-1827
[8] S.B. Liu, Y. Amada, M. Tamura, Y. Nakagawa, K. Tomishige, One-pot selective conversion of furfural into 1, 5-pentanediol over a Pd-added Ir-ReOx/SiO₂ bifunctional catalyst, Green Chem., 16 (2014) 617-626
[9] Y. Nakagawa, S. Liu, M. Tamura, K. Tomishige, Catalytic total hydrodeoxygenation of biomass-derived polyfunctionalized substrates to alkanes, ChemSusChem, 8 (2015) 1114-1132
[10] Y. Nakagawa, M. Tamura, K. Tomishige, Recent development of production technology of diesel-and jet-fuel-range hydrocarbons from inedible biomass, Fuel Process. Technol., 193 (2019) 404-422
[11] S. Bhowmik, S. Darbha, Advances in solid catalysts for selective hydrogenolysis of glycerol to 1, 3-propanediol, Chem. Rev., (2020) 1-65
[12] W. Zhou, Y.J. Zhao, S.P. Wang, X.B. Ma, The effect of metal properties on the reaction routes of glycerol hydrogenolysis over platinum and ruthenium catalysts, Catal. Today, 298 (2017) 2-8
[13] L. Liu, S. Kawakami, Y. Nakagawa, M. Tamura, K. Tomishige, Highly active iridium-rhenium catalyst condensed on silica support for hydrogenolysis of glycerol to 1, 3-propanediol, Appl. Catal. B Environ., 256 (2019) 117775
[14] M. Tamura, Y. Amada, S. Liu, Z. Yuan, Y. Nakagawa, K. Tomishige, Promoting effect of Ru on Ir-ReOx/SiO₂ catalyst in hydrogenolysis of glycerol, J. Mol. Catal. A:Chem., 388 (2014) 177-187
[15] M.J. Pan, J.N. Wang, W.Z. Fu, B.X. Chen, J.Q. Lei, W.Y. Chen, X.Z. Duan, D. Chen, G. Qian, X.G. Zhou, Active sites of Pt/CNTs nanocatalysts for aerobic base-free oxidation of glycerol, Green Energy Environ., 5 (2020) 76-82
[16] Y.Y. Ma, J. Gan, M.J. Pan, Y.F. Zhang, W.Z. Fu, X.Z. Duan, W.Y. Chen, D. Chen, G. Qian, X.G. Zhou, Reaction mechanism and kinetics for Pt/CNTs catalyzed base-free oxidation of glycerol, Chem. Eng. Sci., 203 (2019) 228-236
[17] X.Z. Duan, Y.F. Zhang, M.J. Pan, H. Dong, B.X. Chen, Y.Y. Ma, G. Qian, X.G. Zhou, J. Yang, D. Chen, SbOx-promoted pt nanoparticles supported on CNTs as catalysts for base-free oxidation of glycerol to dihydroxyacetone, AIChE J., 64 (2018) 3979-3987
[18] M. Slinn, K. Kendall, C. Mallon, J. Andrews, Steam reforming of biodiesel by-product to make renewable hydrogen, Bioresour. Technol., 99 (2008) 5851-5858
[19] G.X. Yang, H. Yu, F. Peng, H.J. Wang, J. Yang, D.L. Xie, Thermodynamic analysis of hydrogen generation via oxidative steam reforming of glycerol, Renew. Energ., 36 (2011) 2120-2127
[20] S. Liu, M. Tamura, Z. Shen, Y. Zhang, Y. Nakagawa, K. Tomishige, Hydrogenolysis of glycerol with in-situ produced H₂ by aqueous-phase reforming of glycerol using Pt-modified Ir-ReOx/SiO₂ catalyst, Catal. Today, 303 (2018) 106-116
[21] Y. Nakagawa, Y. Shinmi, S. Koso, K. Tomishige, Direct hydrogenolysis of glycerol into 1, 3-propanediol over rhenium-modified iridium catalyst, J. Catal., 272 (2010) 191-194
[22] C.H. Deng, X.Z. Duan, J.H. Zhou, X.G. Zhou, W.K. Yuan, S.L. Scott, Ir-Re alloy as a highly active catalyst for the hydrogenolysis of glycerol to 1, 3-propanediol, Catal. Sci. Technol., 5 (2015) 1540-1547
[23] W. Zhou, J. Luo, Y. Wang, J.F. Liu, Y.J. Zhao, S.P. Wang, X.B. Ma, WOx domain size, acid properties and mechanistic aspects of glycerol hydrogenolysis over Pt/WOx/ZrO₂, Appl. Catal. B Environ., 242 (2019) 410-421
[24] X.Y. Wan, Q. Zhang, M.M. Zhu, Y. Zhao, Y.M. Liu, C.M. Zhou, Y.H. Yang, Y. Cao, Interface synergy between IrOx and H-ZSM-5 in selective C-O hydrogenolysis of glycerol toward 1, 3-propanediol, J. Catal., 375 (2019) 339-350
[25] C.J. Yang, F. Zhang, N. Lei, M. Yang, F. Liu, Z.L. Miao, Y.N. Sun, X.C. Zhao, A.Q. Wang, Understanding the promotional effect of Au on Pt/WO₃ in hydrogenolysis of glycerol to 1, 3-propanediol, Chinese J. Catal., 39 (2018) 1366-1372
[26] Y. Nakagawa, K. Mori, K. Chen, Y. Amada, M. Tamura, K. Tomishige, Hydrogenolysis of CO bond over Re-modified Ir catalyst in alkane solvent, Appl. Catal. A, 468 (2013) 418-425
[27] Y. Nakagawa, M. Tamura, K. Tomishige, Catalytic materials for the hydrogenolysis of glycerol to 1, 3-propanediol, J. Mater. Chem. A, 2 (2014) 6688-6702
[28] M. Yang, X.C. Zhao, Y.J. Ren, J. Wang, N. Lei, A.Q. Wang, T. Zhang, Pt/Nb-WOx for the chemoselective hydrogenolysis of glycerol to 1, 3-propanediol:Nb dopant pacifying the over-reduction of WOx supports, Chin. J. Catal, 39 (2018) 1027-1037
[29] L.F. Gong, Y. Lu, Y.J. Ding, R.H. Lin, J.W. Li, W.D. Dong, T. Wang, W.M. Chen, Selective hydrogenolysis of glycerol to 1, 3-propanediol over a Pt/WO₃/TiO₂/SiO₂ catalyst in aqueous media, Appl. Catal., A, 390 (2010) 119-126
[30] J.J. Varghese, L.W. Cao, C. Robertson, Y.H. Yang, L.F. Gladden, A.A. Lapkin, S.H. Mushrif, Synergistic contribution of the acidic metal oxide-metal couple and solvent environment in the selective hydrogenolysis of glycerol:A combined experimental and computational study using ReOx-Ir as the catalyst, ACS Catal., 9 (2018) 485-503
[31] K. Tomishige, Y. Nakagawa, M. Tamura, Taming heterogeneous rhenium catalysis for the production of biomass-derived chemicals, Chin. Chem. Lett., 31 (2020) 1071-1077
[32] L.J. Liu, T. Asano, Y. Nakagawa, M. Tamura, K. Okumura, K. Tomishige, Selective Hydrogenolysis of Glycerol to 1, 3-Propanediol over Rhenium-Oxide-Modified Iridium Nanoparticles Coating Rutile Titania Support, ACS Catal., 9 (2019) 10913-10930
[33] X.C. Zhao, J. Wang, M. Yang, N. Lei, L. Li, B.L. Hou, S. Miao, X.L. Pan, A.Q. Wang, T. Zhang, Selective Hydrogenolysis of Glycerol to 1, 3-Propanediol:Manipulating the Frustrated Lewis Pairs by Introducing Gold to Pt/WOx, ChemSusChem, 10 (2017) 819-824
[34] Q.H. Sun, S. Wang, H.C. Liu, Selective hydrogenolysis of glycerol to propylene glycol on supported Pd catalysts:promoting effects of ZnO and mechanistic assessment of active PdZn alloy surfaces, ACS Catal., 7 (2017) 4265-4275
[35] Y.Y. Sun, Z.S. Cai, X.W. Li, P. Chen, Z.Y. Hou, Selective synthesis of 1, 3-propanediol from glycidol over a carbon film encapsulated Co catalyst, Catal. Sci. Technol., 9 (2019) 5022-5030
[36] C.H. Deng, X.Z. Duan, J.H. Zhou, D. Chen, X.G. Zhou, W.K. Yuan, Size effects of Pt-Re bimetallic catalysts for glycerol hydrogenolysis, Catal. Today, 234 (2014) 208-214
[37] C.H. Deng, L. Leng, X.Z. Duan, J.H. Zhou, X.G. Zhou, W.K. Yuan, Support effect on the bimetallic structure of Ir-Re catalysts and their performances in glycerol hydrogenolysis, J. Mol. Catal. A:Chem., 410 (2015) 81-88
[38] Y. Amada, H. Watanabe, Y. Hirai, Y. Kajikawa, Y. Nakagawa, K. Tomishige, Production of biobutanediols by the hydrogenolysis of erythritol, ChemSusChem, 5 (2012) 1991-1999
[39] K. Ye, Z.W. Zhou, J.Q. Shao, L. Lin, D.F. Gao, N. Ta, R. Si, G.X. Wang, X.H. Bao, In Situ Reconstruction of a Hierarchical Sn-Cu/SnOx Core/Shell Catalyst for High-Performance CO₂ Electroreduction, Angew. Chem., Int. Ed., 59 (2020) 4814-4821
[40] X.Y. Long, P. Yin, T. Lei, K.C. Wang, Z.X. Zhan, Methanol electro-oxidation on Cu@Pt/C core-shell catalyst derived from Cu-MOF, Appl. Catal. B Environ., 260 (2020) 118187
[41] S.G. Chen, Z.D. Wei, X.Q. Qi, L.C. Dong, Y.G. Guo, L.J. Wan, Z.G. Shao, L. Li, Nanostructured polyaniline-decorated Pt/C@PANI core-shell catalyst with enhanced durability and activity, J. Am. Chem. Soc., 134 (2012) 13252-13255
[42] K. Chen, K. Mori, H. Watanabe, Y. Nakagawa, K. Tomishige, C-O bond hydrogenolysis of cyclic ethers with OH groups over rhenium-modified supported iridium catalysts, J. Catal., 294 (2012) 171-183
[43] Y.Q. Cao, H. Zhang, S.F. Ji, Z.J. Sui, Z. Jiang, D.S. Wang, F. Zaera, X.G. Zhou, X.Z. Duan, Y.D. Li, Adsorption Site Regulation to Guide Atomic Design of Ni-Ga Catalysts for Acetylene Semi-Hydrogenation, Angew. Chem., 132 (2020) 11744-11749
[44] Y.Q. Cao, Z.J. Sui, Y.A. Zhu, X.G. Zhou, D. Chen, Selective hydrogenation of acetylene over Pd-In/Al₂O₃ catalyst:promotional effect of indium and composition-dependent performance, ACS Catal., 7 (2017) 7835-7846
[45] M. Armbrüster, K. Kovnir, M. Behrens, D. Teschner, Y. Grin, R. Schlögl, Pd-Ga intermetallic compounds as highly selective semihydrogenation catalysts, J. Am. Chem. Soc., 132 (2010) 14745-14747
[46] Y. Amada, H. Watanabe, M. Tamura, Y. Nakagawa, K. Okumura, K. Tomishige, Structure of ReOx Clusters Attached on the Ir Metal Surface in Ir-ReOx/SiO₂ for the Hydrogenolysis Reaction, J. Phys. Chem. C, 116 (2012) 23503-23514
[47] Y. Nakagawa, M. Tamura, K. Tomishige, Perspective on catalyst development for glycerol reduction to C₃ chemicals with molecular hydrogen, Res. Chem. Intermed., 44 (2018) 3879-3903
[48] K. Tomishige, Y. Nakagawa, M. Tamura, Selective hydrogenolysis and hydrogenation using metal catalysts directly modified with metal oxide species, Green Chem., 19 (2017) 2876-2924
[49] H. Yu, Y.P. Jiao, N. Li, J.J. Pang, W.T. Li, X.K. Zhang, X. Li, C.S. Li, Au-CeO₂ Janus-like nanoparticles fabricated by block copolymer templates and their catalytic activity in the degradation of methyl orange, Appl. Surf. Sci., 427 (2018) 771-778
[50] K.A. Kuttiyiel, K. Sasaki, G.-G. Park, M.B. Vukmirovic, L.J. Wu, Y.M. Zhu, J.G. Chen, R.R. Adzic, Janus structured Pt-FeNC nanoparticles as a catalyst for the oxygen reduction reaction, Chem. Commun., 53 (2017) 1660-1663
[51] R. Tang, S. Zhou, jie, C. Li, xia, R. Chen, L. Zhang, yuan, Z. Zhang, wei, L. Yin, wei, Janus-Structured Co-Ti₃C₂ MXene Quantum Dots as a Schottky Catalyst for High-Performance Photoelectrochemical Water Oxidation, Adv. Funct. Mater., 30 (2020) 2000637
[52] Y. Amada, Y. Shinmi, S. Koso, T. Kubota, Y. Nakagawa, K. Tomishige, Reaction mechanism of the glycerol hydrogenolysis to 1, 3-propanediol over Ir-ReOx/SiO₂ catalyst, Appl. Catal. B Environ., 105 (2011) 117-127
[53] K. Tomishige, Y. Nakagawa, M. Tamura, Design of supported metal catalysts modified with metal oxides for hydrodeoxygenation of biomass-related molecules, Curr. Opin. Green. Sustain. Chem., 22 (2020) 13-21
[54] K. Tomishige, M. Tamura, Y. Nakagawa, Role of Re Species and Acid Cocatalyst on Ir-ReOx/SiO₂ in the C-O Hydrogenolysis of Biomass-Derived Substrates, Chem. Rec., 14 (2014) 1041-1054
[55] L. Rout, A. Kumar, R.S. Dhaka, G.N. Reddy, S. Giri, P. Dash, Bimetallic Au-Cu alloy nanoparticles on reduced graphene oxide support:Synthesis, catalytic activity and investigation of synergistic effect by DFT analysis, Appl. Catal., A, 538 (2017) 107-122
[56] G.Y. Bao, J. Bai, C.P. Li, Synergistic effect of the Pd-Ni bimetal/carbon nanofiber composite catalyst in Suzuki coupling reaction, Org. Chem. Front., 6 (2019) 352-361
[57] B. Zugic, L.C. Wang, C. Heine, D.N. Zakharov, B.A. Lechner, E.A. Stach, J. Biener, M. Salmeron, R.J. Madix, C.M. Friend, Dynamic restructuring drives catalytic activity on nanoporous gold-silver alloy catalysts, Nat. Mater., 16 (2017) 558-564
[58] X. Lu, Y.S. Wu, X.L. Yuan, H.L. Wang, An Integrated CO₂ Electrolyzer and Formate Fuel Cell Enabled by a Reversibly Restructuring Pb-Pd Bimetallic Catalyst, Angew. Chem., Int. Ed., 58 (2019) 4031-4035
[59] W.T. Luo, Y. Lyu, L.F. Gong, H. Du, T. Wang, Y.J. Ding, Selective hydrogenolysis of glycerol to 1, 3-propanediol over egg-shell type Ir-ReOx catalysts, RSC Adv., 6 (2016) 13600-13608
[60] S.R. Bare, S.D. Kelly, F. D. Vila, E. Boldingh, E. Karapetrova, J. Kas, G.E. Mickelson, F.S. Modica, N. Yang, J.J. Rehr, Experimental (XAS, STEM, TPR, and XPS) and theoretical (DFT) characterization of supported rhenium catalysts, J. Phys. Chem. C, 115 (2011) 5740-5755
[61] E.L. Kunkes, D.A. Simonetti, J.A. Dumesic, W.D. Pyrz, L.E. Murillo, J.G.G. Chen, D.J. Buttrey, The role of rhenium in the conversion of glycerol to synthesis gas over carbon supported platinum-rhenium catalysts, J. Catal., 260 (2008) 164-177
[62] M. Chia, Y.J. Pagán-Torres, D. Hibbitts, Q.H. Tan, H.N. Pham, A.K. Datye, M. Neurock, R.J. Davis, J.A. Dumesic, Selective hydrogenolysis of polyols and cyclic ethers over bifunctional surface sites on rhodium-rhenium catalysts, J. Am. Chem. Soc., 133 (2011) 12675-12689
[63] Y. Nakagawa, X. Ning, Y. Amada, K. Tomishige, Solid acid co-catalyst for the hydrogenolysis of glycerol to 1, 3-propanediol over Ir-ReOx/SiO₂, Appl. Catal., A, 433 (2012) 128-134
[64] E. Corbos, X. Courtois, N. Bion, P. Marecot, D. Duprez, Impact of the support oxide and Ba loading on the sulfur resistance and regeneration of Pt/Ba/support catalysts, Appl. Catal. B Environ., 80 (2008) 62-71
[65] Y. Deng, L. An, Sulfate accumulation in commercial Pd-Pt/Al₂O₃ and Pt/Al₂O₃ catalysts used for removal of hydrogen from carbon dioxide, Appl. Catal. A, 119 (1994) 13-22
[66] R. Jin, Y. Liu, Z. Wu, H. Wang, T. Gu, Relationship between SO₂ poisoning effects and reaction temperature for selective catalytic reduction of NO over Mn-Ce/TiO₂ catalyst, Catal. Today, 153 (2010) 84-89
[67] Y.Q. Cao, W.Z. Fu, Z.J. Sui, X.Z. Duan, D. Chen, X.G. Zhou, Kinetics Insights and Active Sites Discrimination of Pd-Catalyzed Selective Hydrogenation of Acetylene, Ind. Eng. Chem. Res., 58 (2019) 1888-1895
[68] W.Y. Chen, J. Ji, X. Feng, X.Z. Duan, G. Qian, P. Li, X.G. Zhou, D. Chen, W.K. Yuan, Mechanistic insight into size-dependent activity and durability in Pt/CNT catalyzed hydrolytic dehydrogenation of ammonia borane, J. Am. Chem. Soc., 136 (2014) 16736-16739
[69] M. Shekhar, J. Wang, W. S. Lee, W.D. Williams, S.M. Kim, E.A. Stach, J.T. Miller, W.N. Delgass, F.H. Ribeiro, Size and support effects for the water-gas shift catalysis over gold nanoparticles supported on model Al₂O₃ and TiO₂, J. Am. Chem. Soc., 134 (2012) 4700-4708
[70] F. Zaera, The surface chemistry of metal-based hydrogenation catalysis, ACS Catal., 7 (2017) 4947-4967
[71] M. Haneda, H. Kudo, Y. Nagao, T. Fujitani, H. Hamada, Enhanced activity of Ba-doped Ir/SiO₂ catalyst for NO reduction with CO in the presence of O₂ and SO₂, Catal. Commun., 7 (2006) 423-426
[72] B. Pholjaroen, N. Li, Y.Q. Huang, L. Li, A.Q. Wang, T. Zhang, Selective hydrogenolysis of tetrahydrofurfuryl alcohol to 1, 5-pentanediol over vanadium modified Ir/SiO₂ catalyst, Catal. Today, 245 (2015) 93-99
[73] J.A. Anderson, F.K. Chong, C.H. Rochester, IR study of CO adsorption on Pt, Re and Pt-Re/Al₂O₃ catalysts before and after coking, J. Mol. Catal. A:Chem., 140 (1999) 65-80
[74] S.T. Thompson, H.H. Lamb, Palladium-Rhenium Catalysts for Selective Hydrogenation of Furfural:Evidence for an Optimum Surface Composition, ACS Catal., 6 (2016) 7438-7447
[75] K.G. Azzam, I.V. Babich, K. Seshan, B.L. Mojet, L. Lefferts, Stable and Efficient Pt-Re/TiO₂ catalysts for Water-Gas-Shift:On the Effect of Rhenium, ChemCatChem, 5 (2013) 557-564
[76] F.K. Chong, J.A. Anderson, C.H. Rochester, Effects of Oxidation/Reduction and Oxychlorination/Reduction Cycles on CO Adsorption by Pt-Re/Al₂O₃ Catalysts, J. Catal., 190 (2000) 327-337
[77] W. Daniell, T. Weingand, H. Knözinger, Redox properties of Re₂O₇/Al₂O₃ as investigated by FTIR spectroscopy of adsorbed CO, J. Mol. Catal. A:Chem., 204 (2003) 519-526
[78] B.K. Ly, B. Tapin, M. Aouine, P. Delichere, F. Epron, C. Pinel, C. Especel, M. Besson, Insights into the Oxidation State and Location of Rhenium in Re-Pd/TiO₂ Catalysts for Aqueous-Phase Selective Hydrogenation of Succinic Acid to 1, 4-Butanediol as a Function of Palladium and Rhenium Deposition Methods, ChemCatChem, 7 (2015) 2161-2178
[79] X.Y. She, J. Kwak, Hun, J.M. Sun, J.Z. Hu, M.Y. Hu, C.M. Wang, C.H. Peden, Y. Wang, Highly Dispersed and Active ReOX on Alumina-Modified SBA-15 Silica for 2-Butanol Dehydration, ACS Catal., 2 (2012) 1020-1026
[80] M. Vuurman, D. Stufkens, A. Oskam, I. Wachs, Structural determination of surface rhenium oxide on various oxide supports (Al₂O₃, ZrO₂, TiO₂ and SiO₂), J. Mol. Catal. A:Chem., 76 (1992) 263-285
[81] D.S. Kim, I. Wachs, Surface rhenium oxide-support interaction for supported Re₂O₇ catalysts, J. Catal., 141 (1993) 419-429
[82] S.G. Mueller, P.J. Stallbaumer, D.A. Slade, S.M. Stagg-Williams, Segregation of Pt and Re During CO₂ Reforming of CH₄, Catal. Lett., 103 (2005) 69-74
[83] H. Iida, A. Igarashi, Structure characterization of Pt-Re/TiO₂ (rutile) and Pt-Re/ZrO₂ catalysts for water gas shift reaction at low-temperature, Appl. Catal., A, 303 (2006) 192-198
[84] J.M. Keels, X. Chen, S. Karakalos, C. Liang, J.R. Monnier, J.R. Regalbuto, Aqueous-Phase Hydrogenation of Succinic Acid Using Bimetallic Ir-Re/C Catalysts Prepared by Strong Electrostatic Adsorption, ACS Catal., 8 (2018) 6486-6494
[85] F.F. Tao, S.R. Zhang, L. Nguyen, X.Q. Zhang, Action of bimetallic nanocatalysts under reaction conditions and during catalysis:evolution of chemistry from high vacuum conditions to reaction conditions, Chem. Soc. Rev., 41 (2012) 7980-7993
[86] H.I. Karan, K. Sasaki, K. Kuttiyiel, C.A. Farberow, M. Mavrikakis, R.R. Adzic, Catalytic activity of platinum monolayer on iridium and rhenium alloy nanoparticles for the oxygen reduction reaction, ACS Catal., 2 (2012) 817-824
[87] A. Ruban, H.L. Skriver, J.K. Nørskov, Surface segregation energies in transition-metal alloys, Phys. Rev. B:Condens. Matter Mater. Phys., 59 (1999) 15990

Enhanced recycling performance of bimetallic Ir-Re/SiO₂ catalyst by amberlyst-15 for glycerol hydrogenolysis

Enhanced recycling performance of bimetallic Ir-Re/SiO₂ catalyst by amberlyst-15 for glycerol hydrogenolysis

PDF (PC)

Knowledge

Abstract

Cite this article

share this article

References

Related Articles 3

Recommended Articles

Metrics

Comments

[1]	Qiongna Xiao, Yuyan Jiang, Weiqiang Yuan, Jingjing Chen, Haohong Li, Huidong Zheng. Styrene epoxidation catalyzed by polyoxometalate/quaternary ammonium phase transfer catalysts: The effect of cation size and catalyst deactivation mechanism [J]. Chinese Journal of Chemical Engineering, 2023, 55(3): 192-201.
[2]	Guoxiao Cai, Wei Xiong, Susu Zhou, Pingle Liu, Yang Lv, Fang Hao, Hean Luo, ChangYi Kong. A multi-functional Ru Mo bimetallic catalyst for ultra-efficient C3 alcohols production from liquid phase hydrogenolysis of glycerol [J]. Chinese Journal of Chemical Engineering, 2022, 51(11): 199-215.
[3]	Yuan Wang, Yang Xiao, Guomin Xiao. Sustainable value-added C₃ chemicals from glycerol transformations: A mini review for heterogeneous catalytic processes [J]. Chinese Journal of Chemical Engineering, 2019, 27(7): 1536-1542.