BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B

doi:10.1016/j.cjche.2024.07.004

Chinese Journal of Chemical Engineering ›› 2024, Vol. 74 ›› Issue (10): 31-43.DOI: 10.1016/j.cjche.2024.07.004

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BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B

Hongtao Wang¹, Xiangrui Fan¹, Mingming Yan³, Tianyu Guo^1,2, Xingfa Li¹, Chao Chen², Yu Qi¹

1 College of Environment Science and Engineering, Taiyuan University of Technology, Jinzhong 030600, China;
2 Ministry of Environment Department, China Institute for Radiation Protection, Taiyuan 030006, China;
3 Xinzhou Branch of Petrochina Coalbed Methane Co. Ltd, Xinzhou 036600, China

Received:2024-02-05 Revised:2024-07-06 Accepted:2024-07-08 Online:2024-08-02 Published:2024-10-28
Contact: Chao Chen,E-mail:381450501@qq.com;Yu Qi,E-mail:allstep@163.com
Supported by:
The authors thank the National Natural Science Foundation of China (51572185), Natural Science Foundation of Shanxi Province (202203021211158 and 20210302123176), the Key Research & Development Program of Shanxi Province (Social Development, 201903D321060) and the Key Research & Development program of Shanxi Province (International Cooperation, 201903D421079) for the financial support.

BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B

Hongtao Wang¹, Xiangrui Fan¹, Mingming Yan³, Tianyu Guo^1,2, Xingfa Li¹, Chao Chen², Yu Qi¹

1 College of Environment Science and Engineering, Taiyuan University of Technology, Jinzhong 030600, China;
2 Ministry of Environment Department, China Institute for Radiation Protection, Taiyuan 030006, China;
3 Xinzhou Branch of Petrochina Coalbed Methane Co. Ltd, Xinzhou 036600, China

通讯作者: Chao Chen,E-mail:381450501@qq.com;Yu Qi,E-mail:allstep@163.com
基金资助:
The authors thank the National Natural Science Foundation of China (51572185), Natural Science Foundation of Shanxi Province (202203021211158 and 20210302123176), the Key Research & Development Program of Shanxi Province (Social Development, 201903D321060) and the Key Research & Development program of Shanxi Province (International Cooperation, 201903D421079) for the financial support.

Abstract

Abstract: A series of BiOBr@biomass carbon derived from locust leaves materials (BiOBr@BC) were fabricated and the photocatalytic property was investigated for photocatalytic degradation of rhodamine B (RhB) under visible light. The morphology, structure and photoelectrochemical properties of the photocatalysts were characterized by means of SEM, TEM, XRD, XPS, FT-IR, BET, PL, UV-vis/DRS, and EIS techniques. The results showed that the introduction of BC significantly enhanced the photocatalytic activity. When the content of biomass carbon (BC) in a composite is 3% (based on the mass of BiOBr), the obtained BiOBr@BC-3 exhibits excellent photocatalytic activity, degrading 99% of RhB within 20 min. The excellent degradation efficiency after the introduction of BC can be attributed to the enhanced visible light absorption, narrower band gap, and fast electron-hole pair separation rate. The photocatalytic mechanism on the degradation of RhB was illustrated based on the radicals' trapping experiments and semiconductor energy band position. The proposed material is expected to be of significant application value in the field of wastewater treatment.

Key words: Degradation, Rhodamine B, Adsorption, BiOBr, Renewable energy

摘要： A series of BiOBr@biomass carbon derived from locust leaves materials (BiOBr@BC) were fabricated and the photocatalytic property was investigated for photocatalytic degradation of rhodamine B (RhB) under visible light. The morphology, structure and photoelectrochemical properties of the photocatalysts were characterized by means of SEM, TEM, XRD, XPS, FT-IR, BET, PL, UV-vis/DRS, and EIS techniques. The results showed that the introduction of BC significantly enhanced the photocatalytic activity. When the content of biomass carbon (BC) in a composite is 3% (based on the mass of BiOBr), the obtained BiOBr@BC-3 exhibits excellent photocatalytic activity, degrading 99% of RhB within 20 min. The excellent degradation efficiency after the introduction of BC can be attributed to the enhanced visible light absorption, narrower band gap, and fast electron-hole pair separation rate. The photocatalytic mechanism on the degradation of RhB was illustrated based on the radicals' trapping experiments and semiconductor energy band position. The proposed material is expected to be of significant application value in the field of wastewater treatment.

关键词: Degradation, Rhodamine B, Adsorption, BiOBr, Renewable energy

Hongtao Wang, Xiangrui Fan, Mingming Yan, Tianyu Guo, Xingfa Li, Chao Chen, Yu Qi. BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B[J]. Chinese Journal of Chemical Engineering, 2024, 74(10): 31-43.

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BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B

BiOBr nanosheets coupling with biomass carbon derived from locust leaves for enhanced photocatalytic degradation of rhodamine B

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[3]	Lifang Ge, Meizhen Gao, Xiaosheng Zhang, Jiang Wang, Qi Shi, Jinxiang Dong. Hydrophobic CHA-ZIFs with a junctional trap between cha and d6r cages for adsorption of 2,3-butanediol in aqueous solution [J]. Chinese Journal of Chemical Engineering, 2024, 73(9): 90-100.
[4]	Wenwen Gao, Yuhuan Wang, Wang Li, Zhifang Zhang, Ting Su, Miao Mu, Ying Gong, Rui Dang, Rui Bai, E Zheng, Wei Zhao. A Z-scheme LaFeO₃-CuFe₂O₄ composite for sulfate radical-based photocatalytic process: Synergistic effect and mechanism [J]. Chinese Journal of Chemical Engineering, 2024, 73(9): 256-269.
[5]	Juan Wang, Yanbing Zhu, Zedong Jiang, Xiping Du, Mingjing Zheng, Lijun Li, Hui Ni, Yuanpeng Wang, Zhipeng Li, Qingbiao Li. Characteristics and mechanism of Ni²⁺ and Cd²⁺ adsorption by recovered perlite from agar extraction residue [J]. Chinese Journal of Chemical Engineering, 2024, 72(8): 141-152.
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[10]	B. A. Abdulkadir, R. S. R. Mohd Zaki, A. T. Abd Wahab, S. N. Miskan, Anh-Tam Nguyen, Dai-Viet N. Vo, H. D. Setiabudi. A concise review on surface and structural modification of porous zeolite scaffold for enhanced hydrogen storage [J]. Chinese Journal of Chemical Engineering, 2024, 70(6): 33-53.
[11]	Jing Wen, Ruirui Yuan, Tao Jiang, Tangxia Yu, Yufan Zhang. Solvothermal synthesis and adsorption performance of layered boehmite using aluminum chloride and high-alumina fly ash [J]. Chinese Journal of Chemical Engineering, 2024, 70(6): 280-290.
[12]	Huanxi Xu, Peihua Lin, Pei-Jun Liu, Hai-Gang Liu, Hui-Bin Guo, Chao-Xiang Wu, Ming Fang, Xu Zhang, Guan-Ping Jin. Removal of rubidium from brine by an integrated film of sulfonated polysulfone/graphene/potassium copper ferricyanide [J]. Chinese Journal of Chemical Engineering, 2024, 69(5): 112-121.
[13]	Zhi Hu, Jiahong Wang, Tongtong Sun. Tetraethylenepentamine-functionalized magnetic mesoporous composites as a novel adsorbent for the removal Cr(III)-ethylenediaminetetraacetic acid in complex solution [J]. Chinese Journal of Chemical Engineering, 2024, 68(4): 16-26.
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[15]	Xing Zhong, Yubin Tan, Siyuan Wu, Caixia Hu, Kai Guo, Yongchuan Wu, Neng Yu, Mingyang Ma, Ying Dai. Efficient and rapid capture of uranium(VI) in wastewater via multi-amine modified β-cyclodextrin porous polymer [J]. Chinese Journal of Chemical Engineering, 2024, 68(4): 144-155.