Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation

doi:10.1016/j.cjche.2019.01.001

Chinese Journal of Chemical Engineering ›› 2019, Vol. 27 ›› Issue (6): 1348-1360.DOI: 10.1016/j.cjche.2019.01.001

• Special Issue: Separation Process Intensification of Chemical Engineering • Previous Articles Next Articles

Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation

Ning Zhang¹, Wenxu Qi¹, Lili Huang^1,2, En Jiang¹, Junjiang Bao¹, Xiaopeng Zhang¹, Baigang An², Gaohong He¹

1 State Key Laboratory of Fine Chemicals, School of Petroleum and Chemical Engineering, Dalian University of Technology, Panjin 124221, China;
2 School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051, China

Received:2018-11-30 Revised:2018-12-26 Online:2019-08-19 Published:2019-06-28
Contact: Baigang An, Gaohong He
Supported by:
Supported by the National Natural Science Foundation of China (Grant Nos. 21506019, 51672118, 51672117), the Fundamental Research Funds for the Central Universities (Grant Nos. DUT16RC(4)80, DUT16QY43), the Program for Changjiang Scholars (T2012049).

Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation

Ning Zhang¹, Wenxu Qi¹, Lili Huang^1,2, En Jiang¹, Junjiang Bao¹, Xiaopeng Zhang¹, Baigang An², Gaohong He¹

1 State Key Laboratory of Fine Chemicals, School of Petroleum and Chemical Engineering, Dalian University of Technology, Panjin 124221, China;
2 School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051, China

通讯作者: Baigang An, Gaohong He
基金资助:
Supported by the National Natural Science Foundation of China (Grant Nos. 21506019, 51672118, 51672117), the Fundamental Research Funds for the Central Universities (Grant Nos. DUT16RC(4)80, DUT16QY43), the Program for Changjiang Scholars (T2012049).

Abstract

Abstract: Membrane separation has become an important technology to deal with the global water crisis. The polymerbased membrane technology is currently in the forefront of water purification and desalination but is plagued with some bottlenecks. Laminated graphene oxide (GO) membranes exhibit excellent advantages in water purification and desalination due to the single atomic layer structure, hydrophilic property, rich oxygen-containing groups for modification, mechanical and chemical robust, anti-fouling properties, facile and large-scale production, etc. Thus the GO-based membrane technology is believed to offer huge opportunities for efficient and practical water treatment. This review systematically summarizes the current progress on the water flux and selectivity intensification, stability improvement, anti-fouling and anti-biofouling ability enhancement by structural control and modification. To improve the performance of the laminated GO membrane, interlayer spacing tunability and surface modification are mainly used to enhance its water flux and selectivity. It is found that the stability and biofouling also block the service life of the GO membrane. The crosslinking method is found to effectively solve the stability of GO membrane in aqueous environment. Introducing nanoparticles is a widely used method to improve the membrane biofouling ability. Overall, we believe that this review could provide benefit to researchers in the area of GO-based membrane technology for water treatment.

Key words: Membranes, Graphene oxide, Water flux, Selectivity, Stability, Fouling

摘要： Membrane separation has become an important technology to deal with the global water crisis. The polymerbased membrane technology is currently in the forefront of water purification and desalination but is plagued with some bottlenecks. Laminated graphene oxide (GO) membranes exhibit excellent advantages in water purification and desalination due to the single atomic layer structure, hydrophilic property, rich oxygen-containing groups for modification, mechanical and chemical robust, anti-fouling properties, facile and large-scale production, etc. Thus the GO-based membrane technology is believed to offer huge opportunities for efficient and practical water treatment. This review systematically summarizes the current progress on the water flux and selectivity intensification, stability improvement, anti-fouling and anti-biofouling ability enhancement by structural control and modification. To improve the performance of the laminated GO membrane, interlayer spacing tunability and surface modification are mainly used to enhance its water flux and selectivity. It is found that the stability and biofouling also block the service life of the GO membrane. The crosslinking method is found to effectively solve the stability of GO membrane in aqueous environment. Introducing nanoparticles is a widely used method to improve the membrane biofouling ability. Overall, we believe that this review could provide benefit to researchers in the area of GO-based membrane technology for water treatment.

关键词: Membranes, Graphene oxide, Water flux, Selectivity, Stability, Fouling

Ning Zhang, Wenxu Qi, Lili Huang, En Jiang, Junjiang Bao, Xiaopeng Zhang, Baigang An, Gaohong He. Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation[J]. Chinese Journal of Chemical Engineering, 2019, 27(6): 1348-1360.

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Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation

Review on structural control and modification of graphene oxide-based membranes in water treatment: From separation performance to robust operation

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