SCI和EI收录∣中国化工学会会刊

Chinese Journal of Chemical Engineering ›› 2015, Vol. 23 ›› Issue (8): 1245-1255.DOI: 10.1016/j.cjche.2015.01.012

• 流体力学与传递现象 •    下一篇

A Reynolds mass flux model for gas separation process simulation: II. Application to adsorption on activated carbon in a packed column

Wenbin Li1,2, Kuotsung Yu2, Xigang Yuan2, Botan Liu2   

  1. 1 Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin University, Tianjin 300072, China;
    2 State Key Laboratory for Chemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
  • 收稿日期:2014-01-19 修回日期:2015-01-28 出版日期:2015-08-28 发布日期:2015-09-26
  • 通讯作者: Xigang Yuan
  • 基金资助:

    Supported by the National Natural Science Foundation of China (21376163).

A Reynolds mass flux model for gas separation process simulation: II. Application to adsorption on activated carbon in a packed column

Wenbin Li1,2, Kuotsung Yu2, Xigang Yuan2, Botan Liu2   

  1. 1 Collaborative Innovation Center of Chemical Science and Engineering (Tianjin), Tianjin University, Tianjin 300072, China;
    2 State Key Laboratory for Chemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
  • Received:2014-01-19 Revised:2015-01-28 Online:2015-08-28 Published:2015-09-26
  • Contact: Xigang Yuan
  • Supported by:

    Supported by the National Natural Science Foundation of China (21376163).

摘要: Simulations of adsorption process using the Reynolds mass flux model described in Part I of these serial articles are presented. The object of the simulation is the methylene chloride adsorption in a packed column (0.041mid, packed with spherical activated carbon up to a length of 0.2 m). With the Reynolds mass flux model, breakthrough/regeneration curves, concentration and temperature as well as the velocity distributions can be obtained. The simulated results are compared with the experimental data reported in the literature and satisfactory agreement is found both in breakthrough/regeneration curves and temperature curves. Moreover, the anisotropic turbulent mass diffusion is characterized and discussed.

关键词: Simulation, Adsorption, Mass transfer, Anisotropic turbulent mass diffusion, Packed bed

Abstract: Simulations of adsorption process using the Reynolds mass flux model described in Part I of these serial articles are presented. The object of the simulation is the methylene chloride adsorption in a packed column (0.041mid, packed with spherical activated carbon up to a length of 0.2 m). With the Reynolds mass flux model, breakthrough/regeneration curves, concentration and temperature as well as the velocity distributions can be obtained. The simulated results are compared with the experimental data reported in the literature and satisfactory agreement is found both in breakthrough/regeneration curves and temperature curves. Moreover, the anisotropic turbulent mass diffusion is characterized and discussed.

Key words: Simulation, Adsorption, Mass transfer, Anisotropic turbulent mass diffusion, Packed bed