Facile one-pot synthesis of a BiOBr/Bi2WO6 heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation

doi:10.1016/j.cjche.2022.02.018

Chinese Journal of Chemical Engineering ›› 2023, Vol. 53 ›› Issue (1): 222-231.DOI: 10.1016/j.cjche.2022.02.018

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Facile one-pot synthesis of a BiOBr/Bi₂WO₆ heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation

Duanlian Tang¹, Xiaoyan Chen¹, Jiayan Yan¹, Zhuo Xiong¹, Xiaoyu Lou¹, Changshen Ye¹, Jie Chen^1,2, Ting Qiu¹

1. College of Chemical Engineering, Fuzhou University, Fuzhou 350116, China;
2. College of Environment and Safety Engineering, Fuzhou University, Fuzhou 350108, China

Received:2021-10-18 Revised:2022-01-11 Online:2023-04-08 Published:2023-01-28
Contact: Jie Chen,E-mail:jiechen@fzu.edu.cn;Ting Qiu,E-mail:tingqiu@fzu.edu.cn
Supported by:
We greatly acknowledge the National Natural Science Foundation of China (Grant No. 22108040 and 21878054), the Natural Science Foundation of Fujian Province (2020J05130), Science and Technology Project of Fujian Educational Committee (JAT190051), and Research Project of Ningde Normal University (2019T03).

Facile one-pot synthesis of a BiOBr/Bi₂WO₆ heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation

Duanlian Tang¹, Xiaoyan Chen¹, Jiayan Yan¹, Zhuo Xiong¹, Xiaoyu Lou¹, Changshen Ye¹, Jie Chen^1,2, Ting Qiu¹

1. College of Chemical Engineering, Fuzhou University, Fuzhou 350116, China;
2. College of Environment and Safety Engineering, Fuzhou University, Fuzhou 350108, China

通讯作者: Jie Chen,E-mail:jiechen@fzu.edu.cn;Ting Qiu,E-mail:tingqiu@fzu.edu.cn
基金资助:
We greatly acknowledge the National Natural Science Foundation of China (Grant No. 22108040 and 21878054), the Natural Science Foundation of Fujian Province (2020J05130), Science and Technology Project of Fujian Educational Committee (JAT190051), and Research Project of Ningde Normal University (2019T03).

Abstract

Abstract: Photocatalytic removal of tetracycline (TC) from the wastewater is of great value in the chemical and environmental engineering field. Here, we introduced a facile one-step method for the synthesis of BiOBr/Bi₂WO₆ heterojunctions by using cheap CTAB as the Br source. We showed the possibility of our method to fine-tune the content of BiOBr in the produced BiOBr/Bi₂WO₆ by simply changing the dosage of cetyltrimethylammonium bromide (CTAB), providing a platform for the delicate tuning of the visible-light absorbance ability of the composites. With a suitable heterojunction structure of BiOBr/Bi₂WO₆-0.2, it exhibited an ultrarapid photocatalytic activity towards TC (20 mg·L^-1), with a competitive removal efficiency of 88.1% within 60 min and an ultrahigh removal rate of 0.0349 min^-1. It could also be robustly recycled for at least 5 cycles with slight removal efficiency loss. We demonstrated that this exciting photocatalytic performance was due to the highly decreased recombination of photoinduced electrons and holes on our composites by constructing this heterojunction structure, and the resulting OH and contributed to the effective degradation of TC to CO₂.

Key words: BiOBr/Bi₂WO₆, Heterojunction, Visible light, Photocatalytic, Tetracycline

摘要： Photocatalytic removal of tetracycline (TC) from the wastewater is of great value in the chemical and environmental engineering field. Here, we introduced a facile one-step method for the synthesis of BiOBr/Bi₂WO₆ heterojunctions by using cheap CTAB as the Br source. We showed the possibility of our method to fine-tune the content of BiOBr in the produced BiOBr/Bi₂WO₆ by simply changing the dosage of cetyltrimethylammonium bromide (CTAB), providing a platform for the delicate tuning of the visible-light absorbance ability of the composites. With a suitable heterojunction structure of BiOBr/Bi₂WO₆-0.2, it exhibited an ultrarapid photocatalytic activity towards TC (20 mg·L^-1), with a competitive removal efficiency of 88.1% within 60 min and an ultrahigh removal rate of 0.0349 min^-1. It could also be robustly recycled for at least 5 cycles with slight removal efficiency loss. We demonstrated that this exciting photocatalytic performance was due to the highly decreased recombination of photoinduced electrons and holes on our composites by constructing this heterojunction structure, and the resulting OH and contributed to the effective degradation of TC to CO₂.

关键词: BiOBr/Bi₂WO₆, Heterojunction, Visible light, Photocatalytic, Tetracycline

Duanlian Tang, Xiaoyan Chen, Jiayan Yan, Zhuo Xiong, Xiaoyu Lou, Changshen Ye, Jie Chen, Ting Qiu. Facile one-pot synthesis of a BiOBr/Bi₂WO₆ heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation[J]. Chinese Journal of Chemical Engineering, 2023, 53(1): 222-231.

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Facile one-pot synthesis of a BiOBr/Bi₂WO₆ heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation

Facile one-pot synthesis of a BiOBr/Bi₂WO₆ heterojunction with enhanced visible-light photocatalytic activity for tetracycline degradation

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