Recent progress in porous organic polymers and their application for CO2 capture

doi:10.1016/j.cjche.2021.08.028

Abstract

Abstract: Carbon capture, storage, and utilization (CCSU) is recognized as an effective method to reduce the excessive emission of CO₂. Absorption by amine aqueous solutions is considered highly efficient for CO₂ capture from the flue gas because of the large CO₂ capture capacity and high selectivity. However, it is often limited by the equipment corrosion and the high desorption energy consumption, and adsorption of CO₂ using solid adsorbents has been receiving more attention in recent years due to its simplicity and high efficiency. More recently, a great number of porous organic polymers (POPs) have been designed and constructed for CO₂ capture, and they are proven promising solid adsorbents for CO₂ capture due to their high Brunauer-Emmett-Teller (BET) surface area (S_BET), adjustable pore size and easy functionalization. In particular, they usually have rigid skeleton, permanent porosity, and good physiochemical stability. In this review, we have a detailed review for the different POPs developed in recent years, not only the design strategy, but also the special structure for CO₂ capture. The outlook of the opportunities and challenges of the POPs is also proposed.

Key words: Porous organic polymers, Selectivity, Adsorbent, CO₂ capture

摘要： Carbon capture, storage, and utilization (CCSU) is recognized as an effective method to reduce the excessive emission of CO₂. Absorption by amine aqueous solutions is considered highly efficient for CO₂ capture from the flue gas because of the large CO₂ capture capacity and high selectivity. However, it is often limited by the equipment corrosion and the high desorption energy consumption, and adsorption of CO₂ using solid adsorbents has been receiving more attention in recent years due to its simplicity and high efficiency. More recently, a great number of porous organic polymers (POPs) have been designed and constructed for CO₂ capture, and they are proven promising solid adsorbents for CO₂ capture due to their high Brunauer-Emmett-Teller (BET) surface area (S_BET), adjustable pore size and easy functionalization. In particular, they usually have rigid skeleton, permanent porosity, and good physiochemical stability. In this review, we have a detailed review for the different POPs developed in recent years, not only the design strategy, but also the special structure for CO₂ capture. The outlook of the opportunities and challenges of the POPs is also proposed.

关键词: Porous organic polymers, Selectivity, Adsorbent, CO₂ capture

Jiajia Wang, Lizhi Wang, You Wang, Du Zhang, Qin Xiao, Jianhan Huang, You-Nian Liu. Recent progress in porous organic polymers and their application for CO₂ capture[J]. Chinese Journal of Chemical Engineering, 2022, 42(2): 91-103.

Jiajia Wang, Lizhi Wang, You Wang, Du Zhang, Qin Xiao, Jianhan Huang, You-Nian Liu. Recent progress in porous organic polymers and their application for CO₂ capture[J]. 中国化学工程学报, 2022, 42(2): 91-103.

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Recent progress in porous organic polymers and their application for CO₂ capture

Recent progress in porous organic polymers and their application for CO₂ capture

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