2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS2/CdIn2S4 flower-like heterojunctions

doi:10.1016/j.cjche.2022.04.018

Chinese Journal of Chemical Engineering ›› 2023, Vol. 54 ›› Issue (2): 180-191.DOI: 10.1016/j.cjche.2022.04.018

2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS₂/CdIn₂S₄ flower-like heterojunctions

Qian Zhu¹, Yan Zhuang¹, Hongqing Zhao¹, Peng Zhan¹, Cong Ren¹, Changsheng Su¹, Wenqiang Ren³, Jiawen Zhang¹, Di Cai¹, Peiyong Qin²

1. National Energy R&D Center for Biorefinery, Beijing University of Chemical Technology, Beijing 100029, China;
2. Collage of Life Science and Technology, Beijing University of Chemical Technology, Beijing 100029, China;
3. Research Center for Eco-environmental Sciences, Chinese Academy of Science, Beijing 100085, China

Received:2022-01-18 Revised:2022-03-07 Online:2023-05-11 Published:2023-02-28
Contact: Di Cai,E-mail:caidibuct@163.com;Peiyong Qin,E-mail:qinpeiyong@tsinghua.org.cn
Supported by:
This work was funded by the National Key Research and Development Program of China (2018YFB1501704), the National Natural Science Foundation of China (22078018), and the Beijing Natural Science Foundation (2222016).

2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS₂/CdIn₂S₄ flower-like heterojunctions

Qian Zhu¹, Yan Zhuang¹, Hongqing Zhao¹, Peng Zhan¹, Cong Ren¹, Changsheng Su¹, Wenqiang Ren³, Jiawen Zhang¹, Di Cai¹, Peiyong Qin²

1. National Energy R&D Center for Biorefinery, Beijing University of Chemical Technology, Beijing 100029, China;
2. Collage of Life Science and Technology, Beijing University of Chemical Technology, Beijing 100029, China;
3. Research Center for Eco-environmental Sciences, Chinese Academy of Science, Beijing 100085, China

通讯作者: Di Cai,E-mail:caidibuct@163.com;Peiyong Qin,E-mail:qinpeiyong@tsinghua.org.cn
基金资助:
This work was funded by the National Key Research and Development Program of China (2018YFB1501704), the National Natural Science Foundation of China (22078018), and the Beijing Natural Science Foundation (2222016).

Abstract

Abstract: The selective oxidation of 5-hydroxymethylfurfural (HMF) into 2,5-diformylfuran (DFF) is an important reaction for renewable biomass building blocks. Compared with thermal catalytic processes, photocatalytic production of DFF from HMF has attracted tremendous attention. Herein, the MoS₂/CdIn₂S₄ (MC) flower-like heterojunctions were prepared and considered as photocatalysts for selective oxidation of HMF into DFF under visible-light irradiation in aqueous solution. Results demonstrated MoS₂ in MC heterojunction could promote the separation of photoexcited electron-hole pairs, while the amount of MoS₂ dropping was proved influenced on the photocatalytic performance. 80.93% of DFF selectivity was realized when using 12.5% MC as photocatalyst. In addition, the MC catalyst also showed great potential in transformation of other biomass derived benzyl- and furyl-alcohols. The catalytic mechanism suggested that ·O₂^- was the decisive active radical for HMF oxidation. Therefore, the MC heterojunction could be applied in photocatalytic conversion of biomass to valuable chemicals under ambient condition.

Key words: 2,5-Diformylfuran (DFF), Photocatalysis, MoS₂/CdIn₂S₄ (MC), Selective oxidation, Visible light irradiation

摘要： The selective oxidation of 5-hydroxymethylfurfural (HMF) into 2,5-diformylfuran (DFF) is an important reaction for renewable biomass building blocks. Compared with thermal catalytic processes, photocatalytic production of DFF from HMF has attracted tremendous attention. Herein, the MoS₂/CdIn₂S₄ (MC) flower-like heterojunctions were prepared and considered as photocatalysts for selective oxidation of HMF into DFF under visible-light irradiation in aqueous solution. Results demonstrated MoS₂ in MC heterojunction could promote the separation of photoexcited electron-hole pairs, while the amount of MoS₂ dropping was proved influenced on the photocatalytic performance. 80.93% of DFF selectivity was realized when using 12.5% MC as photocatalyst. In addition, the MC catalyst also showed great potential in transformation of other biomass derived benzyl- and furyl-alcohols. The catalytic mechanism suggested that ·O₂^- was the decisive active radical for HMF oxidation. Therefore, the MC heterojunction could be applied in photocatalytic conversion of biomass to valuable chemicals under ambient condition.

关键词: 2,5-Diformylfuran (DFF), Photocatalysis, MoS₂/CdIn₂S₄ (MC), Selective oxidation, Visible light irradiation

Qian Zhu, Yan Zhuang, Hongqing Zhao, Peng Zhan, Cong Ren, Changsheng Su, Wenqiang Ren, Jiawen Zhang, Di Cai, Peiyong Qin. 2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS₂/CdIn₂S₄ flower-like heterojunctions[J]. Chinese Journal of Chemical Engineering, 2023, 54(2): 180-191.

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2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS₂/CdIn₂S₄ flower-like heterojunctions

2,5-Diformylfuran production by photocatalytic selective oxidation of 5-hydroxymethylfurfural in water using MoS₂/CdIn₂S₄ flower-like heterojunctions

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