Recent advances on the reduction of CO2 to important C2+ oxygenated chemicals and fuels

doi:10.1016/j.cjche.2018.07.008

Chinese Journal of Chemical Engineering ›› 2018, Vol. 26 ›› Issue (11): 2266-2279.DOI: 10.1016/j.cjche.2018.07.008

• Special issue of Carbon Capture, Utilisation and Storage • 上一篇下一篇

Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels

Jiachen Li^1,2,3,4, Liguo Wang^1,3,4, Yan Cao¹, Chanjuan Zhang^1,2,3,4, Peng He¹, Huiquan Li^1,3,4

1 CAS Key Laboratory of Green Process and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China;
2 Chemical and Biochemical Engineering, Technical University of Denmark, DK-2800 Lyngby, Denmark;
3 Sino-Danish College University of Chinese Academy of Sciences, Beijing 100049, China;
4 Sino-Danish Center for Education and Research University of Chinese Academy of Sciences, Beijing 100049, China

收稿日期:2018-05-31 修回日期:2018-07-04 出版日期:2018-11-28 发布日期:2018-12-10
通讯作者: Liguo Wang, Huiquan Li
基金资助:
Supported by the National Natural Science Foundation of China (21576272, 21476244), "Transformational Technologies for Clean Energy and Demonstration", Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDA 21030600), the project from Jiangsu Collaborative Innovation Center for Ecological Building Materials and Environmental Protection Equipment (YCXT201607), and Youth Innovation Promotion Association (2016046) of CAS.

Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels

Jiachen Li^1,2,3,4, Liguo Wang^1,3,4, Yan Cao¹, Chanjuan Zhang^1,2,3,4, Peng He¹, Huiquan Li^1,3,4

1 CAS Key Laboratory of Green Process and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China;
2 Chemical and Biochemical Engineering, Technical University of Denmark, DK-2800 Lyngby, Denmark;
3 Sino-Danish College University of Chinese Academy of Sciences, Beijing 100049, China;
4 Sino-Danish Center for Education and Research University of Chinese Academy of Sciences, Beijing 100049, China

Received:2018-05-31 Revised:2018-07-04 Online:2018-11-28 Published:2018-12-10
Contact: Liguo Wang, Huiquan Li
Supported by:
Supported by the National Natural Science Foundation of China (21576272, 21476244), "Transformational Technologies for Clean Energy and Demonstration", Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDA 21030600), the project from Jiangsu Collaborative Innovation Center for Ecological Building Materials and Environmental Protection Equipment (YCXT201607), and Youth Innovation Promotion Association (2016046) of CAS.

摘要/Abstract

摘要： The chemical utilization of CO₂ is a crucial step for the recycling of carbon resource. In recent years, the study on the conversion of CO₂ into a wide variety of C₂₊ important chemicals and fuels has received considerable attention as an emerging technology. Since CO₂ is thermodynamically stable and kinetically inert, the effective activation of CO₂ molecule for the selective transformation to target products still remains a challenge. The welldesigned CO₂ reduction route and efficient catalyst system has imposed the feasibility of CO₂ conversion into C₂₊ chemicals and fuels. In this paper, we have reviewed the recent advances on chemical conversion of CO₂ into C₂₊ chemicals and fuels with wide practical applications, including important alcohols, acetic acid, dimethyl ether, olefins and gasoline. In particular, the synthetic routes for C-C coupling and carbon chain growth, multifunctional catalyst design and reaction mechanisms are exclusively emphasized.

关键词: CO₂, Reduction, C₂₊, Chemicals, Fuels, Catalysis

Abstract: The chemical utilization of CO₂ is a crucial step for the recycling of carbon resource. In recent years, the study on the conversion of CO₂ into a wide variety of C₂₊ important chemicals and fuels has received considerable attention as an emerging technology. Since CO₂ is thermodynamically stable and kinetically inert, the effective activation of CO₂ molecule for the selective transformation to target products still remains a challenge. The welldesigned CO₂ reduction route and efficient catalyst system has imposed the feasibility of CO₂ conversion into C₂₊ chemicals and fuels. In this paper, we have reviewed the recent advances on chemical conversion of CO₂ into C₂₊ chemicals and fuels with wide practical applications, including important alcohols, acetic acid, dimethyl ether, olefins and gasoline. In particular, the synthetic routes for C-C coupling and carbon chain growth, multifunctional catalyst design and reaction mechanisms are exclusively emphasized.

Key words: CO₂, Reduction, C₂₊, Chemicals, Fuels, Catalysis

Jiachen Li, Liguo Wang, Yan Cao, Chanjuan Zhang, Peng He, Huiquan Li. Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels[J]. Chinese Journal of Chemical Engineering, 2018, 26(11): 2266-2279.

Jiachen Li, Liguo Wang, Yan Cao, Chanjuan Zhang, Peng He, Huiquan Li. Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels[J]. Chin.J.Chem.Eng., 2018, 26(11): 2266-2279.

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Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels

Recent advances on the reduction of CO₂ to important C₂₊ oxygenated chemicals and fuels

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