SCI和EI收录∣中国化工学会会刊

Chinese Journal of Chemical Engineering ›› 2012, Vol. 20 ›› Issue (4): 693-700.

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Effect of Distributor Design on Gas-Liquid Distribution in Monolithic Bed at High Gas/Liquid Ratios

周媛1, AL-DAHHAN Muthanna2, DUDUKOVIC Milorad3, 刘辉1   

  1. 1. Beijing University of Chemical Technology, Beijing 100029, China;
    2. Missouri University of Science and Technology, Rolla, MO 65409, USA;
    3. Washington University in St.Louis, MO 63130, USA
  • 收稿日期:2011-12-11 修回日期:2012-06-21 出版日期:2012-08-28 发布日期:2012-09-15
  • 通讯作者: AL-DAHHAN Muthanna, E-mail:aldahhanm@mst.edu;LIU Hui, E-mail:hliu@mail.buct.edu.cn
  • 基金资助:
    Supported by the State-funded Postgraduates' Overseas Study Program of China Scholarship Council (CSC)

Effect of Distributor Design on Gas-Liquid Distribution in Monolithic Bed at High Gas/Liquid Ratios

ZHOU Yuan1, AL-DAHHAN Muthanna2, DUDUKOVIC Milorad3, LIU Hui1   

  1. 1. Beijing University of Chemical Technology, Beijing 100029, China;
    2. Missouri University of Science and Technology, Rolla, MO 65409, USA;
    3. Washington University in St.Louis, MO 63130, USA
  • Received:2011-12-11 Revised:2012-06-21 Online:2012-08-28 Published:2012-09-15
  • Supported by:
    Supported by the State-funded Postgraduates' Overseas Study Program of China Scholarship Council (CSC)

摘要: Experiments were carried out to investigate the liquid flow distribution at high gas/liquid ratios in a cold model monolith bed of a 0.048 m diameter with 62 cells per cm2.Three types of distributor for the liquid distribution were used to evaluate their distribution performance.Local liquid saturation in individual channels was measured using 16 single-point optical fiber probes mounted inside the channels.The results indicate that 1) The optical fiber probe technique can measure phase distribution in the monolith bed;2) Liquid saturation distribution along the radial direction of the monolith bed is not uniform and the extent of non-uniformity depends on the distributor design and phase velocities;and 3) The tube array distributor provides superior liquid distribution performance over the showerhead and nozzle distributors.

关键词: monolith reactor, phase distribution, optical fiber probe, liquid saturation

Abstract: Experiments were carried out to investigate the liquid flow distribution at high gas/liquid ratios in a cold model monolith bed of a 0.048 m diameter with 62 cells per cm2.Three types of distributor for the liquid distribution were used to evaluate their distribution performance.Local liquid saturation in individual channels was measured using 16 single-point optical fiber probes mounted inside the channels.The results indicate that 1) The optical fiber probe technique can measure phase distribution in the monolith bed;2) Liquid saturation distribution along the radial direction of the monolith bed is not uniform and the extent of non-uniformity depends on the distributor design and phase velocities;and 3) The tube array distributor provides superior liquid distribution performance over the showerhead and nozzle distributors.

Key words: monolith reactor, phase distribution, optical fiber probe, liquid saturation