A route for the study on mass transfer enhancement by adding particles in liquid phase

doi:10.1016/j.cjche.2022.05.013

中国化学工程学报 ›› 2022, Vol. 48 ›› Issue (8): 158-165.DOI: 10.1016/j.cjche.2022.05.013

A route for the study on mass transfer enhancement by adding particles in liquid phase

Xing Su¹, Ning Qiao^2,3, Bao-Chang Sun^2,3

1. College of Chemical and Material Engineering, Quzhou University, Quzhou 324000, China;
2. State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China;
3. Research Center of the Ministry of Education for High Gravity Engineering and Technology, Beijing University of Chemical Technology, Beijing 100029, China

收稿日期:2022-04-01 修回日期:2022-05-27 出版日期:2022-08-28 发布日期:2022-09-30
通讯作者: Bao-Chang Sun,E-mail:sunbc@mail.buct.edu.cn
基金资助:
This work was supported by National Key Research and Development Program of China (2019YFA0210302), the National Natural Science Foundation of China (21878009, 21901141), and Basic Research Plan for Public Welfare of Zhejiang Province, China (LZY21B060001).

A route for the study on mass transfer enhancement by adding particles in liquid phase

Xing Su¹, Ning Qiao^2,3, Bao-Chang Sun^2,3

1. College of Chemical and Material Engineering, Quzhou University, Quzhou 324000, China;
2. State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China;
3. Research Center of the Ministry of Education for High Gravity Engineering and Technology, Beijing University of Chemical Technology, Beijing 100029, China

Received:2022-04-01 Revised:2022-05-27 Online:2022-08-28 Published:2022-09-30
Contact: Bao-Chang Sun,E-mail:sunbc@mail.buct.edu.cn
Supported by:
This work was supported by National Key Research and Development Program of China (2019YFA0210302), the National Natural Science Foundation of China (21878009, 21901141), and Basic Research Plan for Public Welfare of Zhejiang Province, China (LZY21B060001).

摘要/Abstract

摘要： This work presents a route for the study on the absorption performance of gas into liquid under the condition of adding particles in a stirred constant temperature reactor. Two evaluated systems, hydrogen–water and hydrogen–methanol, with the addition of activated carbon particles (ACP) were carried out, respectively. The results showed that the addition of ACP into the water can enhance the mass transfer between hydrogen and water, the enhancement factor increases rapidly with the increase of the ACP content, and then tends to be unchanged. However, for the hydrogen–methanol system, ACP has little effect on the mass transfer performance. In addition, a gas–liquid mass transfer model considering the effect of solid particle enhancement was established based on the shuttle effect and two-film model. Results indicated that the predicted value agreed well with the experimental value in both hydrogen–methanol–ACP and hydrogen–water–ACP systems.

关键词: Mass transfer, Hydrogen, Water, Methanol, Activated carbon

Abstract: This work presents a route for the study on the absorption performance of gas into liquid under the condition of adding particles in a stirred constant temperature reactor. Two evaluated systems, hydrogen–water and hydrogen–methanol, with the addition of activated carbon particles (ACP) were carried out, respectively. The results showed that the addition of ACP into the water can enhance the mass transfer between hydrogen and water, the enhancement factor increases rapidly with the increase of the ACP content, and then tends to be unchanged. However, for the hydrogen–methanol system, ACP has little effect on the mass transfer performance. In addition, a gas–liquid mass transfer model considering the effect of solid particle enhancement was established based on the shuttle effect and two-film model. Results indicated that the predicted value agreed well with the experimental value in both hydrogen–methanol–ACP and hydrogen–water–ACP systems.

Key words: Mass transfer, Hydrogen, Water, Methanol, Activated carbon

Xing Su, Ning Qiao, Bao-Chang Sun. A route for the study on mass transfer enhancement by adding particles in liquid phase[J]. 中国化学工程学报, 2022, 48(8): 158-165.

Xing Su, Ning Qiao, Bao-Chang Sun. A route for the study on mass transfer enhancement by adding particles in liquid phase[J]. Chinese Journal of Chemical Engineering, 2022, 48(8): 158-165.

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A route for the study on mass transfer enhancement by adding particles in liquid phase

A route for the study on mass transfer enhancement by adding particles in liquid phase

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