SCI和EI收录∣中国化工学会会刊

Chinese Journal of Chemical Engineering ›› 2025, Vol. 86 ›› Issue (10): 186-192.DOI: 10.1016/j.cjche.2025.06.017

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Physicochemical properties of UO3 products synthesized via a flame denitrification reactor

Jiaxin Liu1, Mingming Wu2, Qichao Li1, Rui Li1, Lei Li1, Liudong Hou1, Yi Liu2, Jing Ma1   

  1. 1. China Nuclear Power Engineering Co., Ltd., Beijing 100142, China;
    2. School of Chemical Engineering, Dalian University of Technology, Dalian 116024, China
  • Received:2025-03-29 Revised:2025-05-21 Accepted:2025-06-11 Online:2025-08-08 Published:2025-10-28
  • Contact: Liudong Hou,E-mail:hould@cnpe.cc;Yi Liu,E-mail:diligenliu@dlut.edu.cn;Jing Ma,E-mail:majing@cnpe.cc
  • Supported by:
    The authors are grateful to Xing Yuan Program of China National Nuclear Corporation (CNPE-8208) and National Natural Science Foundation of China (22478056) for the financial support.

Physicochemical properties of UO3 products synthesized via a flame denitrification reactor

Jiaxin Liu1, Mingming Wu2, Qichao Li1, Rui Li1, Lei Li1, Liudong Hou1, Yi Liu2, Jing Ma1   

  1. 1. China Nuclear Power Engineering Co., Ltd., Beijing 100142, China;
    2. School of Chemical Engineering, Dalian University of Technology, Dalian 116024, China
  • 通讯作者: Liudong Hou,E-mail:hould@cnpe.cc;Yi Liu,E-mail:diligenliu@dlut.edu.cn;Jing Ma,E-mail:majing@cnpe.cc
  • 基金资助:
    The authors are grateful to Xing Yuan Program of China National Nuclear Corporation (CNPE-8208) and National Natural Science Foundation of China (22478056) for the financial support.

Abstract: The rational utilization of nuclear energy is crucial in current global energy system. Using a flame denitrification reactor, this study develops uranium trioxide (UO3), a critical intermediate product in the nuclear fuel cycle, and systematically characterizes its physicochemical properties. The UO3 products are comprehensively examined to assess their suitability for downstream nuclear industry applications. Our results indicates that high-quality UO3 products can be obtained using flame denitrification reactor at temperatures between 440 °C and 480 °C. This study reveals the considerable potential of UO3 production via flame denitrification, marking a significant advancement towards enhanced nuclear fuel cycle systems.

Key words: Flame denitrification reactor, Uranium trioxide synthesis, Nuclear fuel cycle, Chemical processes, Thermodynamics

摘要: The rational utilization of nuclear energy is crucial in current global energy system. Using a flame denitrification reactor, this study develops uranium trioxide (UO3), a critical intermediate product in the nuclear fuel cycle, and systematically characterizes its physicochemical properties. The UO3 products are comprehensively examined to assess their suitability for downstream nuclear industry applications. Our results indicates that high-quality UO3 products can be obtained using flame denitrification reactor at temperatures between 440 °C and 480 °C. This study reveals the considerable potential of UO3 production via flame denitrification, marking a significant advancement towards enhanced nuclear fuel cycle systems.

关键词: Flame denitrification reactor, Uranium trioxide synthesis, Nuclear fuel cycle, Chemical processes, Thermodynamics