SCI和EI收录∣中国化工学会会刊

中国化学工程学报 ›› 2020, Vol. 28 ›› Issue (11): 2707-2722.DOI: 10.1016/j.cjche.2020.07.037

• Review •    下一篇

A review on single bubble gas–liquid mass transfer

Yuyun Bao, Jinting Jia, Shuaifei Tong, Zhengming Gao, Ziqi Cai   

  1. State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China
  • 收稿日期:2019-11-29 修回日期:2020-07-20 出版日期:2020-11-28 发布日期:2020-12-31
  • 通讯作者: Zhengming Gao, Ziqi Cai
  • 基金资助:
    This work was supported by the National Key Research & Development Program of China (2017YFB0306703), the National Natural Science Foundation of China (No. 21676007) and the Fundamental Research Funds for the Central Universities (XK1802-1).

A review on single bubble gas–liquid mass transfer

Yuyun Bao, Jinting Jia, Shuaifei Tong, Zhengming Gao, Ziqi Cai   

  1. State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China
  • Received:2019-11-29 Revised:2020-07-20 Online:2020-11-28 Published:2020-12-31
  • Contact: Zhengming Gao, Ziqi Cai
  • Supported by:
    This work was supported by the National Key Research & Development Program of China (2017YFB0306703), the National Natural Science Foundation of China (No. 21676007) and the Fundamental Research Funds for the Central Universities (XK1802-1).

摘要: It is common to empirically correlate volumetric mass transfer coefficient kLa for predicting gas-liquid mass transfer in industrial applications, and the investigation of single bubble mass transfer is crucial for a detailed understanding of mass transfer mechanism. In this work, experiments, models and simulations based on the experimental results were highlighted to elucidate the mass transfer between single bubbles and ambient liquid. The experimental setups, measurement methods, the mass transfer of single bubbles in the Newtonian and the nonNewtonian liquid, models derived from the concept of eddy diffusion, the extension of Whitman's, Higbie's and Danckwerts' models, or dimensionless numbers, and simulation methods on turbulence, gas-liquid partition methods and mass transfer source term determination are introduced and commented on. Although people have a great knowledge on mass transfer between single bubbles and ambient liquid in single conditions, it is still insufficient when facing complex liquid conditions or some phenomena such as turbulence, contamination or non-Newtonian behavior. Additional studies on single bubbles are required for experiments and models in various liquid conditions in future.

关键词: Gas-liguid mass transfer, Single bubbles, Mass transfer models, Simulation, Surfactant, Non-Newtonian fluid

Abstract: It is common to empirically correlate volumetric mass transfer coefficient kLa for predicting gas-liquid mass transfer in industrial applications, and the investigation of single bubble mass transfer is crucial for a detailed understanding of mass transfer mechanism. In this work, experiments, models and simulations based on the experimental results were highlighted to elucidate the mass transfer between single bubbles and ambient liquid. The experimental setups, measurement methods, the mass transfer of single bubbles in the Newtonian and the nonNewtonian liquid, models derived from the concept of eddy diffusion, the extension of Whitman's, Higbie's and Danckwerts' models, or dimensionless numbers, and simulation methods on turbulence, gas-liquid partition methods and mass transfer source term determination are introduced and commented on. Although people have a great knowledge on mass transfer between single bubbles and ambient liquid in single conditions, it is still insufficient when facing complex liquid conditions or some phenomena such as turbulence, contamination or non-Newtonian behavior. Additional studies on single bubbles are required for experiments and models in various liquid conditions in future.

Key words: Gas-liguid mass transfer, Single bubbles, Mass transfer models, Simulation, Surfactant, Non-Newtonian fluid