SCI和EI收录∣中国化工学会会刊

中国化学工程学报 ›› 2022, Vol. 44 ›› Issue (4): 321-331.DOI: 10.1016/j.cjche.2021.03.006

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Fluidization dynamic characteristics of carbon nanotube particles in a tapered fluidized bed

Wenjuan Bai, Dianming Chu, Yan He   

  1. Shandong Engineering Laboratory for Preparation and Application of High-performance Carbon-Materials, College of Electromechanical Engineering, Qingdao University of Science and Technology, Shandong 266061, China
  • 收稿日期:2020-09-16 修回日期:2021-03-02 出版日期:2022-04-28 发布日期:2022-06-18
  • 通讯作者: Yan He,E-mail:heyan@qust.edu.cn
  • 基金资助:
    This work is supported by the National Natural Science Foundation of China (51676103) and Taishan Scholar Project of Shandong Province (ts20190937).

Fluidization dynamic characteristics of carbon nanotube particles in a tapered fluidized bed

Wenjuan Bai, Dianming Chu, Yan He   

  1. Shandong Engineering Laboratory for Preparation and Application of High-performance Carbon-Materials, College of Electromechanical Engineering, Qingdao University of Science and Technology, Shandong 266061, China
  • Received:2020-09-16 Revised:2021-03-02 Online:2022-04-28 Published:2022-06-18
  • Contact: Yan He,E-mail:heyan@qust.edu.cn
  • Supported by:
    This work is supported by the National Natural Science Foundation of China (51676103) and Taishan Scholar Project of Shandong Province (ts20190937).

摘要: In this work, a tapered fluidized bed (TFB) without a distributor for fluidizing carbon nanotube (CNT) was applied for improving the dead zone, blockage, and fracture of distributor, which occurred in actual production. Experiments were performed under different superficial gas velocities, static bed heights, CNT agglomerate size, and positions of pressure probe. To obtain multi-perspective and multi-scale understanding of fluidization dynamics of gas–CNT flow in the TFB without a distributor, the standard deviation, skewness, kurtosis, wavelet decompositions and homogeneous index analysis methods were adopted. Some noticeable phenomena were observed. Particle movements including inter-particle, gas–particle and particle–wall dominate dynamic characteristics. The amplitudes of pressure fluctuations of coarse agglomerated multi-walled CNT were more sensitive to the gas velocity than that of fine agglomerated multi-walled CNT. The sensitively of energy contribution of the meso- and macro-structures was that the sensitivity of the measured position was less than the sensitivity of the energy contribution by the changes of particle size, and the sensitivity of the energy contribution by the changes of particle size was less than the energy contribution by the changes of gas velocity. The fluidization quality of coarse agglomerated multi-walled CNT was better than that of fine agglomerated multi-walled CNT, which was verified by the skewness and wavelet analysis.

关键词: Tapered fluidized bed, Gas–CNT flow, Pressure fluctuation, Wavelet, Homogeneous index, Carbon nanotubes

Abstract: In this work, a tapered fluidized bed (TFB) without a distributor for fluidizing carbon nanotube (CNT) was applied for improving the dead zone, blockage, and fracture of distributor, which occurred in actual production. Experiments were performed under different superficial gas velocities, static bed heights, CNT agglomerate size, and positions of pressure probe. To obtain multi-perspective and multi-scale understanding of fluidization dynamics of gas–CNT flow in the TFB without a distributor, the standard deviation, skewness, kurtosis, wavelet decompositions and homogeneous index analysis methods were adopted. Some noticeable phenomena were observed. Particle movements including inter-particle, gas–particle and particle–wall dominate dynamic characteristics. The amplitudes of pressure fluctuations of coarse agglomerated multi-walled CNT were more sensitive to the gas velocity than that of fine agglomerated multi-walled CNT. The sensitively of energy contribution of the meso- and macro-structures was that the sensitivity of the measured position was less than the sensitivity of the energy contribution by the changes of particle size, and the sensitivity of the energy contribution by the changes of particle size was less than the energy contribution by the changes of gas velocity. The fluidization quality of coarse agglomerated multi-walled CNT was better than that of fine agglomerated multi-walled CNT, which was verified by the skewness and wavelet analysis.

Key words: Tapered fluidized bed, Gas–CNT flow, Pressure fluctuation, Wavelet, Homogeneous index, Carbon nanotubes