Recent developments and consideration issues in solid adsorbents for CO2 capture from flue gas

doi:10.1016/j.cjche.2018.07.012

Chinese Journal of Chemical Engineering ›› 2018, Vol. 26 ›› Issue (11): 2303-2317.DOI: 10.1016/j.cjche.2018.07.012

• Special issue of Carbon Capture, Utilisation and Storage • 上一篇下一篇

Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas

Lijuan Nie^1,2, Yuanyuan Mu^1,2, Junsu Jin¹, Jian Chen², Jianguo Mi¹

1 Beijing Key Laboratory of Membrane Science and Technology, Beijing University of Chemical Technology, Beijing 100029, China;
2 State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China

收稿日期:2018-05-31 修回日期:2018-07-11 出版日期:2018-11-28 发布日期:2018-12-10
通讯作者: Junsu Jin, Jian Chen
基金资助:
Supported by the National Key Research & Development Program of China (2017YFB0603302).

Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas

Lijuan Nie^1,2, Yuanyuan Mu^1,2, Junsu Jin¹, Jian Chen², Jianguo Mi¹

1 Beijing Key Laboratory of Membrane Science and Technology, Beijing University of Chemical Technology, Beijing 100029, China;
2 State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China

Received:2018-05-31 Revised:2018-07-11 Online:2018-11-28 Published:2018-12-10
Contact: Junsu Jin, Jian Chen
Supported by:
Supported by the National Key Research & Development Program of China (2017YFB0603302).

摘要/Abstract

摘要： The increase in energy demand caused by industrialization leads to abundant CO₂ emissions into atmosphere and induces abrupt rise in earth temperature. It is vital to acquire relatively simple and cost-effective technologies to separate CO₂ from the flue gas and reduce its environmental impact. Solid adsorption is now considered an economic and least interfering way to capture CO₂, in that it can accomplish the goal of small energy penalty and few modifications to power plants. In this regard, we attempt to review the CO₂ adsorption performances of several types of solid adsorbents, including zeolites, clays, activated carbons, alkali metal oxides and carbonates, silica materials, metal-organic frameworks, covalent organic frameworks, and polymerized high internal phase emulsions. These solid adsorbents have been assessed in their CO₂ adsorption capacities along with other important parameters including adsorption kinetics, effect of water, recycling stability and regenerability. In particular, the superior properties of adsorbents enhanced by impregnating or grafting amine groups have been discussed for developing applicable candidates for industrial CO₂ capture.

关键词: CO₂ capture, Adsorption, Adsorbents, Inorganic materials, Organic materials

Abstract: The increase in energy demand caused by industrialization leads to abundant CO₂ emissions into atmosphere and induces abrupt rise in earth temperature. It is vital to acquire relatively simple and cost-effective technologies to separate CO₂ from the flue gas and reduce its environmental impact. Solid adsorption is now considered an economic and least interfering way to capture CO₂, in that it can accomplish the goal of small energy penalty and few modifications to power plants. In this regard, we attempt to review the CO₂ adsorption performances of several types of solid adsorbents, including zeolites, clays, activated carbons, alkali metal oxides and carbonates, silica materials, metal-organic frameworks, covalent organic frameworks, and polymerized high internal phase emulsions. These solid adsorbents have been assessed in their CO₂ adsorption capacities along with other important parameters including adsorption kinetics, effect of water, recycling stability and regenerability. In particular, the superior properties of adsorbents enhanced by impregnating or grafting amine groups have been discussed for developing applicable candidates for industrial CO₂ capture.

Key words: CO₂ capture, Adsorption, Adsorbents, Inorganic materials, Organic materials

Lijuan Nie, Yuanyuan Mu, Junsu Jin, Jian Chen, Jianguo Mi. Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas[J]. Chinese Journal of Chemical Engineering, 2018, 26(11): 2303-2317.

Lijuan Nie, Yuanyuan Mu, Junsu Jin, Jian Chen, Jianguo Mi. Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas[J]. Chin.J.Chem.Eng., 2018, 26(11): 2303-2317.

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Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas

Recent developments and consideration issues in solid adsorbents for CO₂ capture from flue gas

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