A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures

doi:10.1016/j.cjche.2020.03.033

中国化学工程学报 ›› 2021, Vol. 29 ›› Issue (1): 383-390.DOI: 10.1016/j.cjche.2020.03.033

• Resources and Environmental Technology • 上一篇下一篇

A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures

Zhenqiang Zhang¹, Danfeng Yu¹, Xiubin Xu¹, Huayi Li², Taoyan Mao¹, Cheng Zheng¹, Jianjia Huang¹, Hui Yang³, Zihan Niu¹, Xu Wu¹

1 School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China;
2 CAS Key Lab of Engineering Plastics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China;
3 CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China

收稿日期:2020-02-03 修回日期:2020-03-24 出版日期:2021-01-28 发布日期:2021-04-02
通讯作者: Danfeng Yu, Xu Wu
基金资助:
We wish to thank the National Natural Science Foundations of China (Nos. 21878059, 21878058, 21808044), the Science and Technology Project of Guangdong Province (2017A050501040), the Science and Technology Project of the Guangzhou Education Bureau (201831830, 201831825) for sponsoring this research.

A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures

Zhenqiang Zhang¹, Danfeng Yu¹, Xiubin Xu¹, Huayi Li², Taoyan Mao¹, Cheng Zheng¹, Jianjia Huang¹, Hui Yang³, Zihan Niu¹, Xu Wu¹

1 School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China;
2 CAS Key Lab of Engineering Plastics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China;
3 CAS Key Lab of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China

Received:2020-02-03 Revised:2020-03-24 Online:2021-01-28 Published:2021-04-02
Contact: Danfeng Yu, Xu Wu
Supported by:
We wish to thank the National Natural Science Foundations of China (Nos. 21878059, 21878058, 21808044), the Science and Technology Project of Guangdong Province (2017A050501040), the Science and Technology Project of the Guangzhou Education Bureau (201831830, 201831825) for sponsoring this research.

摘要/Abstract

摘要： Porous materials with selective wettability and permeability have significant importance in oil-water separation, but complex fabrication processes are typically required to obtain the desired structures with suitable surface chemistry. In this work, an industrial melt-blown strategy that utilized commercially available polypropylene (PP) was used for the large-scale fabrication of superhydrophobic/superoleophilic membranes with staggered fabric structures. These membranes could readily separate different oils including pump oil and crude oil from various aqueous solutions such as strongly acidic, alkaline, and saline media. In addition, the separation efficiencies of these membranes exceeded 99%, and they could remain functional even after exposure to corrosive media. We anticipate that this work will further the design of membranes and enhance their applicability in oil-water separation, and provide researchers and engineers with a more effective tool for performing challenging separations and mitigating pollution.

关键词: Separation, Polypropylene membranes, Surface, Superhydrophobicity, Superoleophilicity, Environment

Abstract: Porous materials with selective wettability and permeability have significant importance in oil-water separation, but complex fabrication processes are typically required to obtain the desired structures with suitable surface chemistry. In this work, an industrial melt-blown strategy that utilized commercially available polypropylene (PP) was used for the large-scale fabrication of superhydrophobic/superoleophilic membranes with staggered fabric structures. These membranes could readily separate different oils including pump oil and crude oil from various aqueous solutions such as strongly acidic, alkaline, and saline media. In addition, the separation efficiencies of these membranes exceeded 99%, and they could remain functional even after exposure to corrosive media. We anticipate that this work will further the design of membranes and enhance their applicability in oil-water separation, and provide researchers and engineers with a more effective tool for performing challenging separations and mitigating pollution.

Key words: Separation, Polypropylene membranes, Surface, Superhydrophobicity, Superoleophilicity, Environment

Zhenqiang Zhang, Danfeng Yu, Xiubin Xu, Huayi Li, Taoyan Mao, Cheng Zheng, Jianjia Huang, Hui Yang, Zihan Niu, Xu Wu. A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures[J]. 中国化学工程学报, 2021, 29(1): 383-390.

参考文献

[1] M.A. Shannon, P.W. Bohn, M. Elimelech, J.G. Georgiadis, B.J. Marinas, A.M. Mayes, Science and technology for water purification in the coming decades, Nature 452(2008) 301-310.
[2] A.K. Kota, G. Kwon, W. Choi, J.M. Mabry, A. Tuteja, Hygro-responsive membranes for effective oil-water separation, Nat. Commun. 3(2012) 1-8.
[3] J.J. Huang, D.F. Yu, X.B. Xu, M.H. Liu, Z.Q. Ye, G. Yang, T. Chen, H. Yang, J.B. Wang, X. Wu, Ultra-high flux and efficient oil-water separation via polymer-based electrophoretic deposition, Chem. Eng. J. 371(2019) 575-582.
[4] R.K. Gupta, G.J. Dunderdale, M.W. England, A. Hozumi, Oil/water separation techniques:A review of recent progresses and future directions, J. Mater. Chem. A 5(2017) 16025-16058.
[5] V.T. Tran, X.B. Xu, M.T.I. Mredha, J.X. Cui, J.J. Vlassak, I. Jeon, Hydrogel bowls for cleaning oil spills on water, Water Res. 145(2018) 640-649.
[6] X. Wu, Y.C. Zhang, M.H. Liu, X.B. Xu, Z.P. Wang, I. Wyman, H. Yang, F.H. Liu, J.B. Wang, J.Z. Wu, Preventing crude oil adhesion using fully waterborne coatings, AIChE J. 65(2019), e16569.
[7] W.F. Zhang, N. Liu, Y.Z. Cao, X. Lin, Y.A. Liu, L. Feng, Superwetting porous materials for wastewater treatment:From immiscible oil/water mixture to emulsion separation, Adv. Mater. Interfaces 4(2017) 1600029.
[8] J.S. Eow, M. Ghadiri, A.O. Sharif, T.J. Williams, Electrostatic enhancement of coalescence of water droplets in oil:A review of the current understanding, Chem. Eng. J. 84(2001) 173-192.
[9] A. Al-Shamrani, A. James, H. Xiao, Destabilisation of oil-water emulsions and separation by dissolved air flotation, Water Res. 36(2002) 1503-1512.
[10] H. Yoon, S.H. Na, J.Y. Choi, S.S. Latthe, M.T. Swihart, S.S. Al-Deyab, S.S. Yoon, Gravitydriven hybrid membrane for oleophobic-superhydrophilic oil-water separation and water purification by graphene, Langmuir 30(2014) 11761-11769.
[11] S. Oh, S. Ki, S. Ryu, M.C. Shin, J. Lee, C. Lee, Y. Nam, Performance analysis of gravitydriven oil-water separation using membranes with special wettability, Langmuir 35(2019) 7769-7782.
[12] Y.L. Yu, H. Chen, Y. Liu, V.S.J. Craig, Z.P. Lai, Selective separation of oil and water with mesh membranes by capillarity, Adv. Colloid Interf. Sci. 235(2016) 46-55.
[13] X. Feng, L. Jiang, Design and creation of superwetting/antiwetting surfaces, Adv. Mater. 18(2006) 3063-3078.
[14] J. Ge, H.Y. Zhao, H.W. Zhu, J. Huang, L.A. Shi, S.H. Yu, Advanced sorbents for oil-spill cleanup:Recent advances and future perspectives, Adv. Mater. 28(2016) 10459.
[15] Y.Z. Zhu, D. Wang, L. Jiang, J. Jin, Recent progress in developing advanced membranes for emulsified oil/water separation, NPG Asia Mater. 6(2014), e101.
[16] H.J. Cao, W.H. Gu, J.Y. Fu, Y. Liu, S.G. Chen, Preparation of superhydrophobic/oleophilic copper mesh for oil-water separation, Appl. Surf. Sci. 412(2017) 599-605.
[17] J.Y. Huang, S.H. Li, M.Z. Ge, L.N. Wang, T.L. Xing, G.Q. Chen, X.F. Liu, S.S. Al-Deyab, K.Q. Zhang, T. Chen, Y.K. Lai, Robust superhydrophobic TiO₂@fabrics for UV shielding, self-cleaning and oil-water separation, J. Mater. Chem. A 3(2015) 2825-2832.
[18] J. Li, L. Yan, X.H. Tang, H. Feng, D.C. Hu, F. Zha, Robust superhydrophobic fabric bag filled with polyurethane sponges used for vacuum-assisted continuous and ultrafast absorption and collection of oils from water, Adv. Mater. Interfaces 3(2016) 1500770.
[19] X.J. Yue, Z.D. Li, T. Zhang, D.Y. Yang, F.X. Qiu, Design and fabrication of superwetting fiber-based membranes for oil/water separation applications, Chem. Eng. J. 364(2019) 292-309.
[20] H.C. Yang, K.J. Liao, H. Huang, Q.Y. Wu, L.S. Wan, Z.K. Xu, Mussel-inspired modification of a polymer membrane for ultra-high water permeability and oil-in-water emulsion separation, J. Mater. Chem. A 2(2014) 10225-10230.
[21] S.U. Patel, G.G. Chase, Separation of water droplets from water-in-diesel dispersion using superhydrophobic polypropylene fibrous membranes, Sep. Purif. Technol. 126(2014) 62-68.
[22] Y.Y. Ren, J.N. Guo, Q. Lu, D. Xu, J. Qin, F. Yan, Polypropylene nonwoven fabric@poly (ionic liquid)s for switchable oil/water separation, dye absorption, and antibacterial applications, ChemSusChem 11(2018) 1092-1098.
[23] X. Wu, I. Wyman, G.W. Zhang, J. Lin, Z.Q. Liu, Y. Wang, H. Hu, Preparation of superamphiphobic polymer-based coatings via spray-and dip-coating strategies, Prog. Org. Coat. 90(2016) 463-471.
[24] G.H. Jiang, R.B. Hu, X.H. Wang, X.G. Xi, R.J. Wang, Z. Wei, X. Li, B.L. Tang, Preparation of superhydrophobic and superoleophilic polypropylene fibers with application in oil/water separation, J. Text. Inst. 104(2013) 790-797.
[25] Z.L. Xu, K. Miyazaki, T. Hori, Fabrication of polydopamine-coated superhydrophobic fabrics for oil/water separation and self-cleaning, Appl. Surf. Sci. 370(2016) 243-251.
[26] A.M. Kansara, S.G. Chaudhri, P.S. Singh, A facile one-step preparation method of recyclable superhydrophobic polypropylene membrane for oil-water separation, RSC Adv. 6(2016) 61129-61136.
[27] M.H. Liu, D.F. Yu, X.B. Xu, H. Yang, I. Wyman, J.B. Wang, X. Wu, Endowing recyclability to anti-adhesion materials via designing physically crosslinked polyurethane, J. Mater. Chem. A 7(2019) 22903-22911.
[28] J. Li, R.M. Kang, X.H. Tang, H.D. She, Y.X. Yang, F. Zha, Superhydrophobic meshes that can repel hot water and strong corrosive liquids used for efficient gravity-driven oil/water separation, Nanoscale 8(2016) 7638-7645.
[29] T.Y. Zhao, D.M. Zhang, C.M. Yu, L. Jiang, Facile fabrication of a polyethylene mesh for oil/water separation in a complex environment, ACS Appl. Mater. Interfaces 8(2014) 24186-24191.
[30] S. Bano, U. Zulfiqar, U. Zaheer, M. Awais, I. Ahmad, T. Subhani, Durable and recyclable superhydrophobic fabric and mesh for oil-water separation, Adv. Eng. Mater. 20(2018) 1700460.
[31] K.L. Jin, S.S. Kim, J. Xu, F.S. Bates, C. Ellison, Melt-blown cross-linked fibers from thermally reversible Diels-Alder polymer networks, ACS Macro Lett. 7(2018) 1339-1345.
[32] L. Liu, Z.H. Xu, C.Y. Song, Q.B. Gu, Y.M. Sang, G.L. Lu, H.L. Hu, F.S. Li, Adsorption-filtration characteristics of melt-blown polypropylene fiber in purification of reclaimed water, Desalination 201(2006) 198-206.
[33] S.H. Li, J.Y. Huang, Z. Chen, G.Q. Chen, Y.K. Lai, A review on special wettability textiles:theoretical models, fabrication technologies and multifunctional applications, J. Mater. Chem. A 5(2017) 31-55.
[34] X.D. Zhang, X.L. Wang, X.H. Liu, C.J. Lv, Y.M. Wang, G.Q. Zheng, H. Liu, C.T. Liu, Z.H. Guo, C.Y. Shen, Porous polyethylene bundles with enhanced hydrophobicity and pumping oil-recovery ability via skin-peeling, ACS Sustain. Chem. Eng. 6(2018) 12580-12585.
[35] Y.Z. Cao, X.Y. Zhang, L. Tao, K. Li, Z.X. Xue, L. Feng, Y. Wei, Mussel-inspired chemistry and michael addition reaction for efficient oil/water separation, ACS Appl. Mater. Interfaces 5(2013) 4438-4442.
[36] W.X. Li, W.H. Xing, N.P. Xu, Modeling of relationship between water permeability and microstructure parameters of ceramic membranes, Desalination 192(2006) 340-345.
[37] A. García, S. Álvarez, F. Riera, R. Álvarez, J. Coca, Water and hexane permeate flux through organic and ceramic membranes:effect of pretreatment on hexane permeate flux, J. Membr. Sci. 253(2005) 139-147.
[38] S.K. Mah, C.C.H. Chang, T.Y. Wu, S.P. Chai, The study of reverse osmosis on glycerin solution filtration:Dead-end and crossflow filtrations, transport mechanism, rejection and permeability investigations, Desalination 352(2014) 66-81.
[39] L. Kang, J.P. Li, J.S. Zeng, W.H. Gao, J. Xu, Z. Cheng, K.F. Chen, B. Wang, Water solventassisted condensation polymerization strategy of the superhydrophobic lignocellulosic fiber for efficient oil/water separation, J. Mater. Chem. A 7(2019) 16447-16457.
[40] W.J. Ma, M.J. Zhang, Z.C. Liu, M.M. Kang, C.B. Huang, G.D. Fu, Fabrication of highly durable and robust superhydrophobic-superoleophilic nanofibrous membranes based on a fluorine-free system for efficient oil/water separation, J. Membr. Sci. 570(2019) 303-313.
[41] X.J. Liu, L. Ge, W. Li, X.Z. Wang, F. Li, Layered double hydroxide functionalized textile for effective oil/water separation and selective oil adsorption, ACS Appl. Mater. Interfaces 7(2015) 791-800.
[42] X.Y. Zhou, Z.Z. Zhang, X.H. Xu, F. Guo, X.T. Zhu, X.H. Men, B. Ge, Robust and durable superhydrophobic cotton fabrics for oil/water separation, ACS Appl. Mater. Interfaces 5(2013) 7208-7214.
[43] H. Huang, M. Liu, Y. Li, Y. Yu, X.Z. Yin, J. Wu, S.H. Chen, J. Xu, L.X. Wang, H. Wang, Polyphenylene sulfide microfiber membrane with superhydrophobicity and superoleophilicity for oil/water separation, J. Mater. Sci. 53(2018) 13243-13252.
[44] M.J. Zhang, W.J. Ma, S.T. Wu, G.S. Tang, J.X. Cui, Q.L. Zhang, F. Chen, R.H. Xiong, C.B. Huang, Electrospun frogspawn structured membrane for gravity-driven oil-water separation, J. Colloid Interface Sci. 547(2019) 136-144.
[45] J. Drabek, M. Zatloukal, M. Martyn, Effect of molecular weight on secondary Newtonian plateau at high shear rates for linear isotactic melt blown polypropylenes, J. Non-New. Fl. Mech. 251(2018) 107-118.

A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures

A polypropylene melt-blown strategy for the facile and efficient membrane separation of oil-water mixtures

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价

[1]	Pan Wang, Mengdei Zhou, Zhuangxin Wei, Lu Liu, Tao Cheng, Xiaohua Tian, Jianming Pan. Preparation of bowl-shaped polydopamine surface imprinted polymer composite adsorbent for specific separation of 2′-deoxyadenosine[J]. 中国化学工程学报, 2023, 60(8): 69-79.
[2]	Peipei Ai, Huiqing Jin, Jie Li, Xiaodong Wang, Wei Huang. Ultra-stable Cu-based catalyst for dimethyl oxalate hydrogenation to ethylene glycol[J]. 中国化学工程学报, 2023, 60(8): 186-193.
[3]	Wenwen Zhang, Zhigang Xue, Liyun Cui, Haoliang Gao, Di Zhao, Rongfei Zhou, Weihong Xing. Synthesis of an IMF zeolite membrane for the separation of xylene isomer[J]. 中国化学工程学报, 2023, 60(8): 205-211.
[4]	Hammad Saulat, Jianhua Yang, Tao Yan, Waseem Raza, Wensen Song, Gaohong He. Tungsten incorporated mobil-type eleven zeolite membranes: Facile synthesis and tuneable wettability for highly efficient separation of oil/water mixtures[J]. 中国化学工程学报, 2023, 60(8): 242-252.
[5]	Yuan Liu, Hanting Xiong, Jingwen Chen, Shixia Chen, Zhenyu Zhou, Zheling Zeng, Shuguang Deng, Jun Wang. One-step ethylene separation from ternary C₂ hydrocarbon mixture with a robust zirconium metal-organic framework[J]. 中国化学工程学报, 2023, 59(7): 9-15.
[6]	Hui Jiang, Zijian Zhao, Ning Yu, Yi Qin, Zhengwei Luo, Wenhua Geng, Jianliang Zhu. Synthesis, characterization, and performance comparison of boron using adsorbents based on N-methyl-D-glucosamine[J]. 中国化学工程学报, 2023, 59(7): 16-31.
[7]	Borui Liu, Tao Zhang, Yi Zheng, Kailong Li, Hui Pan, Hao Ling. A dynamic control structure of liquid-only transfer stream distillation column[J]. 中国化学工程学报, 2023, 59(7): 135-145.
[8]	Yafei Su, Xuke Zhang, Hui Li, Donglai Peng, Yatao Zhang. In-situ incorporation of halloysite nanotubes with 2D zeolitic imidazolate framework-L based membrane for dye/salt separation[J]. 中国化学工程学报, 2023, 58(6): 103-111.
[9]	Shuangtai Liu, Lei He, Qiuxiang Yao, Xi Li, Linyang Wang, Jing Wang, Ming Sun, Xiaoxun Ma. Separation and analysis of six fractions in low temperature coal tar by column chromatography[J]. 中国化学工程学报, 2023, 58(6): 256-265.
[10]	Wende Tian, Jiawei Zhang, Zhe Cui, Haoran Zhang, Bin Liu. Microscopic mechanism study and process optimization of dimethyl carbonate production coupled biomass chemical looping gasification system[J]. 中国化学工程学报, 2023, 58(6): 291-305.
[11]	Yanli Zhang, Zhengkun Hou, Dong Yao, Xiaomin Qiu, Hongru Zhang, Peizhe Cui, Yinglong Wang, Jun Gao, Zhaoyou Zhu, Limei Zhong. Energy, exergy, economic and environmental comprehensive analysis and multi-objective optimization of a sustainable zero liquid discharge integrated process for fixed-bed coal gasification wastewater[J]. 中国化学工程学报, 2023, 58(6): 341-354.
[12]	Haike Li, Xindong Li, Guozai Ouyang, Lang Li, Zhaohuang Zhong, Meng Cai, Wenhao Li, Wanfu Huang. Tannic acid/Fe³⁺ interlayer for preparation of high-permeability polyetherimide organic solvent nanofiltration membranes for organic solvent separation[J]. 中国化学工程学报, 2023, 57(5): 17-29.
[13]	Bin Lin, Wenyao Chen, Nan Song, Zhihua Zhang, Qianhong Wang, Wei Du, Xinggui Zhou, Xuezhi Duan. Mechanistic insights into propylene oxidation to acrolein over gold catalysts[J]. 中国化学工程学报, 2023, 57(5): 39-49.
[14]	Hui Yi Leong, Xiao-Qian Fu, Xiang-Yu Liu, Shan-Jing Yao, Dong-Qiang Lin. Characterisation and separation of infectious bursal disease virus-like particles using aqueous two-phase systems[J]. 中国化学工程学报, 2023, 57(5): 72-78.
[15]	Linlin Su, Meijun Chen, Li Gong, Hua Yang, Chao Chen, Jun Wu, Ling Luo, Gang Yang, Lulu Long. Boost activation of peroxymonosulfate by iron doped K_2-xMn₈O₁₆: Mechanism and properties[J]. 中国化学工程学报, 2023, 57(5): 88-97.