In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method

doi:10.1016/j.cjche.2020.07.032

中国化学工程学报 ›› 2021, Vol. 33 ›› Issue (5): 286-296.DOI: 10.1016/j.cjche.2020.07.032

• Resources and Environmental Technology • 上一篇下一篇

In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method

Lei Ma¹, Hongxia Lv¹, Haonan Yu¹, Lingtong Kong¹, Rongyue Zhang¹, Xiaoyan Guo¹, Haibo Jin¹, Guangxiang He¹, Xiaoyan Liu²

1 Beijing Key Laboratory of Fuels Cleaning and Advanced Catalytic Emission Reduction Technology, College of Chemical Engineering, Beijing Institute of Petrochemical Technology, Beijing 102617,;
China;
2 Water Resource Office of Jining City, Shandong Province, Jining 272019, China

收稿日期:2020-03-20 修回日期:2020-07-09 出版日期:2021-05-28 发布日期:2021-08-19
通讯作者: Haibo Jin, Guangxiang He
基金资助:
This work was funded by Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges under Beijing Municipality (IDHT20180508), Scientific Research Common Program of Beijing Municipal Commission of Education (KM202010017006), the Talents Project of Beijing Organization Department (2018000020124G091), the Strategic Priority Research Program of the Chinese Academy of Sciences (XDA21021101) and the National Key Research and Development Program of China (2019YFA0705803).

In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method

Lei Ma¹, Hongxia Lv¹, Haonan Yu¹, Lingtong Kong¹, Rongyue Zhang¹, Xiaoyan Guo¹, Haibo Jin¹, Guangxiang He¹, Xiaoyan Liu²

1 Beijing Key Laboratory of Fuels Cleaning and Advanced Catalytic Emission Reduction Technology, College of Chemical Engineering, Beijing Institute of Petrochemical Technology, Beijing 102617,;
China;
2 Water Resource Office of Jining City, Shandong Province, Jining 272019, China

Received:2020-03-20 Revised:2020-07-09 Online:2021-05-28 Published:2021-08-19
Contact: Haibo Jin, Guangxiang He
Supported by:
This work was funded by Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges under Beijing Municipality (IDHT20180508), Scientific Research Common Program of Beijing Municipal Commission of Education (KM202010017006), the Talents Project of Beijing Organization Department (2018000020124G091), the Strategic Priority Research Program of the Chinese Academy of Sciences (XDA21021101) and the National Key Research and Development Program of China (2019YFA0705803).

摘要/Abstract

摘要： A series of high oil-absorption resins with low cross-linking degree were synthesized by suspension polymerization using stearyl methacrylate (SMA), 2-Ethylhexyl methacrylate (EHMA), and styrene (St) as monomers. Response surface methodology (RSM) with central composite design (CCD) was also applied to determine the optimal parameters that are mainly known to affect their synthesis. Thus, the effects of the monomer mass ratio (EHMA:SMA), the rigid monomer (St) dosage, the porous agent (acetone) dosage, and their pairwise interaction on the resin's oil-absorption capacity were analyzed, highlighting PSES-R2 as the resin with the optimum performance. The pure oil-absorption rates of PSES-R₂ for gasoline, diesel, and kerosene were 11.19 g·g^-1, 16.25 g·g^-1, and 14.84 g·g^-1, respectively, while the oil removal rates from oily wastewater were 98.82%, 65.11%, and 99.63%, respectively.

关键词: Oil-absorption resin, Response surface method, Oil removal rate, Waste water, Absorption, Polymerization

Abstract: A series of high oil-absorption resins with low cross-linking degree were synthesized by suspension polymerization using stearyl methacrylate (SMA), 2-Ethylhexyl methacrylate (EHMA), and styrene (St) as monomers. Response surface methodology (RSM) with central composite design (CCD) was also applied to determine the optimal parameters that are mainly known to affect their synthesis. Thus, the effects of the monomer mass ratio (EHMA:SMA), the rigid monomer (St) dosage, the porous agent (acetone) dosage, and their pairwise interaction on the resin's oil-absorption capacity were analyzed, highlighting PSES-R2 as the resin with the optimum performance. The pure oil-absorption rates of PSES-R₂ for gasoline, diesel, and kerosene were 11.19 g·g^-1, 16.25 g·g^-1, and 14.84 g·g^-1, respectively, while the oil removal rates from oily wastewater were 98.82%, 65.11%, and 99.63%, respectively.

Key words: Oil-absorption resin, Response surface method, Oil removal rate, Waste water, Absorption, Polymerization

Lei Ma, Hongxia Lv, Haonan Yu, Lingtong Kong, Rongyue Zhang, Xiaoyan Guo, Haibo Jin, Guangxiang He, Xiaoyan Liu. In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method[J]. 中国化学工程学报, 2021, 33(5): 286-296.

参考文献

[1] X. Yu, Z. Wang, J. Liu, H. Mei, D. Yong, J. Li, Preparation, swelling behaviors and fertilizer-release properties of sodium humate modified superabsorbent resin, Mater. Today Commun. 19(2019) 124-130.
[2] L. Kong, L. Ma, H. Jin, J. Hou, G. He, R. Zhang, Synthesis of a novel oil-absorption resin and optimization of its performance parameters using response surface design, Polym. Adv. Technol. 30(6) (2019) 1441-1452.
[3] Y. Du, P. Fang, J. Chen, X. Hou, Synthesis of reusable macroporous St/BMA copolymer resin and its absorbency to organic solvent and oil, Polym. Adv. Technol. 27(3) (2016) 393-403.
[4] R. Nasiri, N. Arsalani, Y. Panahian, One-pot synthesis of novel magnetic three-dimensional graphene/chitosan/nickel ferrite nanocomposite for lead ions removal from aqueous solution: RSM modelling design, J. Clean. Prod. 201(2018) 507-515.
[5] E. Rafiee, E. Noori, A. Zinatizadeh, H. Zanganeh, A new visible driven nanocomposite including Ti-substituted polyoxometalate/TiO₂: Synthesis, characterization, photodegradation of azo dye process optimization by RSM and specific removal rate calculations, J. Mater. Sci-Mater El. 29(24) (2018) 20668-20679.
[6] N. Ji, H. Chen, M. Yu, R. Qu, C. Wang, Synthesis of high oil-absorption resins of poly (methyl methacrylate-butyl methacrylate) by suspended emulsion polymerization, Polym. Adv. Technol. 22(12) (2011) 1898-1904.
[7] J. Sun, Y. Xu, H. Chen, Z. Tan, L. Fan, Synthesis and properties of high oil-absorbing resins with long chain by high internal phase emulsions as template, Sep. Sci. Technol. 49(16) (2014) 2518-2524.
[8] J. Wang, Y. Zheng, A. Wang, Preparation and oil absorbency of kapok-g-butyl methacrylate, Environ. Technol. 39(9) (2018) 1089-1095.
[9] Y. Duan, F. Bian, H. Huang, Facile fabrication of porous oil-absorbent microspheres with high oil absorbency and fast oil absorption speed, Polym. Adv. Technol. 27(2) (2016) 228-234.
[10] M. Mäkelä, Experimental design and response surface methodology in energy applications: A tutorial review, Energ. Convers. Manage. 151(2017) 630-640.
[11] Z. Li, L. Shao, W. Hu, T. Zheng, L. Lu, Y. Cao, Excellent reusable chitosan/cellulose aerogel as an oil and organic solvent absorbent, Carbohydr. Polym. 191(2018) 183-190.
[12] M.O. Adebajo, R.L. Frost, J.T. Kloprogge, O. Carmody, S. Kokot, Porous materials for Oil Spill Cleanup: A review of synthesis and absorbing properties, J. Porous. Mater. 12(2003) 159-170.
[13] Y. Neolaka, G. Supriyanto, H. Kusuma, Synthesis and characterization of natural zeolite with ordered ion imprinted polymer structures (IIP@AFINZ) for selective Cr (VI) adsorption from aqueous solution, Mor. J. Chem. 7(2019) 194-210.
[14] A. Diraki, H. Mackey, G. McKay, A. Abdala, Removal of emulsified and dissolved diesel oil from high salinity wastewater by adsorption onto graphene oxide, J. Environ. Chem. Eng. 7(3) (2019) 103106.
[15] S. Songsaeng, P. Thamyongkit, S. Poompradub, Natural rubber/reduced-graphene oxide composite materials: Morphological and oil adsorption properties for treatment of oil spills, J. Adv. Res. 20(2019) 79-89.
[16] Y. Neolaka, Z. Ngara, Y. Lawa, J. Naat, D. Benu, A. Chetouani, H. Elmsellem, H. Darmokoesoemo, H. Kusuma, Simple design and preliminary evaluation of continuous submerged solid small-scale laboratory photoreactor (CS4PR) using TiO₂/NO³-@TC for dye degradation, J. Environ. Chem. Eng. 7(6) (2019) 103482.
[17] Y. Neolaka, Y. Lawa, J. Naat, A. Riwu, H. Darmokoesoemo, G. Supriyanto, C. Holdsworth, A. Amenaghawon, H. Kusuma, A Cr(VI)-imprinted-poly(4-VP-coEGDMA) sorbent prepared using precipitation polymerization and its application for selective adsorptive removal and solid phase extraction of Cr(VI) ions from electroplating industrial wastewater, React. Funct. Polym. 147(2020) 104451.
[18] T. Zhang, Z. Li, Y. Lü, Y. Liu, D. Yang, Q. Li, F. Qiu, Recent progress and future prospects of oil-absorbing materials, Chin. J. Chem. Eng. 27(6) (2020) 1282-1295.

In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method

In-depth investigation on the factors affecting the performance of high oil-absorption resin by response surface method

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价

[1]	Bo Yu, Guang Fu, Xinpei Li, Libo Zhang, Jing Li, Hongtao Qu, Dongbin Wang, Qingfeng Dong, Mengmeng Zhang. Arsenic removal from acidic industrial wastewater by ultrasonic activated phosphorus pentasulfide[J]. 中国化学工程学报, 2023, 60(8): 46-52.
[2]	Yanli Zhang, Zhengkun Hou, Dong Yao, Xiaomin Qiu, Hongru Zhang, Peizhe Cui, Yinglong Wang, Jun Gao, Zhaoyou Zhu, Limei Zhong. Energy, exergy, economic and environmental comprehensive analysis and multi-objective optimization of a sustainable zero liquid discharge integrated process for fixed-bed coal gasification wastewater[J]. 中国化学工程学报, 2023, 58(6): 341-354.
[3]	Yutong Jiang, Yifeng Chen, Fuliu Yang, Jixue Fan, Jun Li, Zhuhong Yang, Xiaoyan Ji. Efficient SO₂ removal using aqueous ionic liquid at low partial pressure[J]. 中国化学工程学报, 2023, 58(6): 355-363.
[4]	Haike Li, Xindong Li, Guozai Ouyang, Lang Li, Zhaohuang Zhong, Meng Cai, Wenhao Li, Wanfu Huang. Tannic acid/Fe³⁺ interlayer for preparation of high-permeability polyetherimide organic solvent nanofiltration membranes for organic solvent separation[J]. 中国化学工程学报, 2023, 57(5): 17-29.
[5]	Linlin Su, Meijun Chen, Li Gong, Hua Yang, Chao Chen, Jun Wu, Ling Luo, Gang Yang, Lulu Long. Boost activation of peroxymonosulfate by iron doped K_2-xMn₈O₁₆: Mechanism and properties[J]. 中国化学工程学报, 2023, 57(5): 88-97.
[6]	Yongbo Liu, Zhihao Si, Cong Ren, Hanzhu Wu, Peng Zhan, Yuqing Peng, Peiyong Qin. Ultrathin polyamide nanofiltration membrane prepared by triazine-based porous organic polymer as interlayer for dye removal[J]. 中国化学工程学报, 2023, 57(5): 193-201.
[7]	Feng Pan, Sugang Ma, Yu Ge, Chuanlin Fan, Qingshan Zhu. Fluidization thermal decomposition of sodium fluosilicate[J]. 中国化学工程学报, 2023, 57(5): 329-337.
[8]	Wen Tian, Junyi Ji, Hongjiao Li, Changjun Liu, Lei Song, Kui Ma, Siyang Tang, Shan Zhong, Hairong Yue, Bin Liang. Measurements of the effective mass transfer areas for the gas–liquid rotating packed bed[J]. 中国化学工程学报, 2023, 55(3): 13-19.
[9]	Bowen Jiang, Jia Liu, Guoqiang Yang, Zhibing Zhang. Efficient conversion of CO₂ into cyclic carbonates under atmospheric by halogen and metal-free poly(ionic liquid)s[J]. 中国化学工程学报, 2023, 55(3): 202-211.
[10]	Yuandong Cui, Bin He, Yu Lei, Yu Liang, Wanting Zhao, Jian Sun, Xiaomin Liu. Lignin derived absorbent for efficient and sustainable CO₂ capture[J]. 中国化学工程学报, 2023, 54(2): 89-97.
[11]	Yilin Song, Yize Zhang, Hao Zhou. Experimental study on the desulfurization and evaporation characteristics of Ca(OH)₂ droplets[J]. 中国化学工程学报, 2023, 54(2): 127-135.
[12]	Aiqin Gao, Xiang Luo, Huanghuang Chen, Aiqin Hou, Hongjuan Zhang, Kongliang Xie. Design of the reactive dyes containing large planar multi-conjugated systems and their application in non-aqueous dyeing[J]. 中国化学工程学报, 2023, 54(2): 264-271.
[13]	Xiaodong Yang, Na Yang, Ziqiang Gong, Feifei Peng, Bin Jiang, Yongli Sun, Luhong Zhang. The superhydrophobic sponge decorated with Ni-Co double layered oxides with thiol modification for continuous oil/water separation[J]. 中国化学工程学报, 2023, 54(2): 296-305.
[14]	Honggui Han, Meiting Sun, Huayun Han, Xiaolong Wu, Junfei Qiao. Univariate imputation method for recovering missing data in wastewater treatment process[J]. 中国化学工程学报, 2023, 53(1): 201-210.
[15]	Jing Gao, Zhijun Ma, Fuli Liu, Cunxin Chen. Synthesis of carbon-coated cobalt ferrite core–shell structure composite: A method for enhancing electromagnetic wave absorption properties by adjusting impedance matching[J]. 中国化学工程学报, 2022, 47(7): 206-217.