Effects of Gas Temperature Fluctuation on the Soot Formation Reactions

doi:10.1016/S1004-9541(13)60437-1

Chinese Journal of Chemical Engineering ›› 2013, Vol. 21 ›› Issue (1): 25-30.DOI: 10.1016/S1004-9541(13)60437-1

Effects of Gas Temperature Fluctuation on the Soot Formation Reactions

陈莹, 张健

Department of Engineering Mechanics, Tsinghua University, Beijing 100084, China

收稿日期:2011-08-24 修回日期:2012-07-12 出版日期:2013-02-28 发布日期:2013-02-04
通讯作者: ZHANG Jian
基金资助:
Supported jointly by the National Natural Science Foundation of China (51076082) and the State Key Laboratory of Engines (SKLE200902).

Effects of Gas Temperature Fluctuation on the Soot Formation Reactions

CHEN Ying, ZHANG Jian

Department of Engineering Mechanics, Tsinghua University, Beijing 100084, China

Received:2011-08-24 Revised:2012-07-12 Online:2013-02-28 Published:2013-02-04
Supported by:
Supported jointly by the National Natural Science Foundation of China (51076082) and the State Key Laboratory of Engines (SKLE200902).

摘要/Abstract

摘要： The effects of gas temperature fluctuations on soot formation and oxidation reactions are investigated numerically in a reacting flow. The instantaneous variations of soot mass fraction with time are obtained under the time-averaged gas temperature of 1500-1700 K. The simulation results show that the gas temperature fluctuation has obvious influence on the instantaneous processes of soot formation and oxidation. Within the present range of gas temperature, the gas temperature fluctuation results in generally lower soot mass fraction comparing to that without gas temperature fluctuation. The increase in the fluctuation amplitude of gas temperature leads to decrease in time-averaged soot mass fraction and increase in time-averaged soot particle number density.

关键词: gas temperature fluctuation, soot formation, reacting flow, numerical simulation

Abstract: The effects of gas temperature fluctuations on soot formation and oxidation reactions are investigated numerically in a reacting flow. The instantaneous variations of soot mass fraction with time are obtained under the time-averaged gas temperature of 1500-1700 K. The simulation results show that the gas temperature fluctuation has obvious influence on the instantaneous processes of soot formation and oxidation. Within the present range of gas temperature, the gas temperature fluctuation results in generally lower soot mass fraction comparing to that without gas temperature fluctuation. The increase in the fluctuation amplitude of gas temperature leads to decrease in time-averaged soot mass fraction and increase in time-averaged soot particle number density.

Key words: gas temperature fluctuation, soot formation, reacting flow, numerical simulation

陈莹, 张健 . Effects of Gas Temperature Fluctuation on the Soot Formation Reactions[J]. Chinese Journal of Chemical Engineering, 2013, 21(1): 25-30.

CHEN Ying, ZHANG Jian. Effects of Gas Temperature Fluctuation on the Soot Formation Reactions[J]. Chin.J.Chem.Eng., 2013, 21(1): 25-30.

参考文献

1 Gomez, A., Littman, M.G., Glassman, I., “Comparative study of soot formation on the centerline of axisymmetric laminar diffusion flames: Fuel and temperature effects”, Combust. Flame, 70, 225-241 (1987).

2 Sunderland, P.B., Faeth, G.M., “Soot formation in hydrocarbon/air laminar jet diffusion flames”, Combust. Flame, 105, 132-146 (1996).

3 Roditcheva, O.V., Bai, X.S., “Pressure effect on soot formation in turbulent diffusion flames”, Chemosphere, 42, 811-821 (2001).

4 Bockhorn, H., “A short introduction to the problem-structure of the following parts”, In: Soot Formation in Combustion, Bockhorn, H., ed., Springer-Verlag, Berlin, 3-7 (1994).

5 Frenklach, M., Wang, H., “Detailed modeling of soot particle nucleation and growth”, Proc. Combust. Inst., 23, 1559-1566 (1990).

6 Frenklach, M., Wang, H., “Detailed mechanism and modeling of soot particle formation”, In: Soot Formation in Combustion, Bockhorn, H., ed., Springer-Verlag, Berlin, 165-192 (1994).

7 Mauss, F., Schafer, T., Bockhorn, H., “Inception and growth of soot particles in dependence on the surrounding gas phase”, Combust. Flame, 99, 697-705 (1994).

8 Leung, K.M., Lindstedt, R.P., Jones, W.P., “A simplified reaction mechanism for soot formation in nonpremixed flames”, Combust. Flame, 87, 289-305 (1991).

9 Lindstedt, P.R., “Simplified soot nucleation and surface growth steps for non-premixed flames”, In: Soot Formation in Combustion, Bockhorn, H., ed., Springer-Verlag, Berlin, 417-441 (1994).

10 Kennedy, I.M., Yam, C., Rapp, D.C., Santoro, R.J., “Modeling and measurements of soot and species in a laminar diffusion flame”, Combust. Flame, 107, 368-382 (1996).

11 Brookes, S.J., Moss, J.B., “Predictions of soot and thermal radiation properties in confined turbulent jet diffusion flames”, Combust. Flame, 116, 486-503 (1999).

12 Liu, F., Guo, H., Smallwood, G.J., Gülder, Ö.L., “Numerical modelling of soot formation and oxidation in laminar coflow non-smoking and smoking ethylene diffusion flames”, Combust. Theory Modelling, 7, 301-315 (2003).

13 Liu, F., Thomson, K.A., Guo, H., Smallwood, G.J., “Numerical and experimental study of an axisymmetric coflow laminar methane-air diffusion flame at pressures between 5 and 40 atmospheres”, Combust. Flame, 146, 456-471 (2006).

14 Zhang, Y., Zhou, H., Xie, M., Fang, Q., Wei, Y., “Modeling of soot formation in gas burner using reduced chemical kinetics coupled with CFD code”, Chin. J. Chem. Eng., 18, 967-978 (2010).

15 Harris, S.J., Weiner, A.M., “Determination of the rate constant for soot surface growth”, Combust. Sci. Technol., 32, 267-275 (1983).

16 Vandsburger, U., Kennedy, I., Glassman, I., “Sooting counterflow diffusion flames with varying oxygen index”, Combust. Sci. Technol., 39, 263-285 (1984).

17 Garo, A., Prado, G., Lahaye J., “Chemical aspects of soot particles oxidation in a laminar methane-air diffusion flame”, Combust. Flame, 79, 226-233 (1990).

18 Ma, G., Wen, J.Z., Lightstone, M.F., Thomson, M.J., “Optimization of soot modeling in turbulent nonpremixed ethylene/air jet flames”, Combust. Sci. Technol., 177, 1567-1602 (2005).

19 Patankar, S.V., Numerical Heat Transfer and Fluid Flow, Hemisphere Publishing Corporation, Washington DC (1980).

20 Hedman, P.O., Warren, D.L., “Turbulent velocity and temperature measurements from a gas-fueled technology combustor with a practical fuel injector”, Combust. Flame, 100, 185-192 (1995).

21 Smoot, L.D., Smith, P.J., Coal Combustion and Gasification, Plenum Press, New York (1985).

22 Megaridis, C.M., Dobbins, R.A., “Comparison of soot growth and oxidation in smoking and non-smoking ethylene diffusion flames”, Combust. Sci. Technol., 66, 1-16 (1989).

23 Dobbins, R.A., Subramaniasivam, H., “Soot precursor particles in flames”, In: Soot Formation in Combustion, Bockhorn, H., ed., Springer-Verlag, Berlin, 290-301 (1994).

24 Said, R., Garo, A., Borghi, R., “Soot formation modeling for turbulent flames”, Combust. Flame, 108, 71-86 (1997).

25 McEnally, C.S., Pfefferle, L.D., “Experimental study of nonfuel hydrocarbons and soot in coflowing partially premixed ethylene/air flames”, Combust. Flame, 121, 575-592 (2000).

26 Hwang, J.Y., Chung, S.H., “Growth of soot particles in counterflow diffusion flames of ethylene”, Combust. Flame, 125, 752-762 (2001).

[1]	Jiahao Xing, Huaizhi Han, Ruitian Yu, Wen Luo. Numerical simulation of flow and heat transfer of n-decane in sub-millimeter spiral tube at supercritical pressure[J]. 中国化学工程学报, 2023, 60(8): 173-185.
[2]	Jian Han, Xinhua Liu, Shanwei Hu, Nan Zhang, Jingjing Wang, Bin Liang. Optimization of decoupling combustion characteristics of coal briquettes and biomass pellets in household stoves[J]. 中国化学工程学报, 2023, 59(7): 182-192.
[3]	Shengfeng Luo, Song Zhang, Yiping Zeng, Hui Zhang, Lili Zheng, Zhaopeng Xu. Study on oxygen transport and titanium oxidation in coating cracks under parallel gas flow based on LBM modelling[J]. 中国化学工程学报, 2023, 56(4): 15-24.
[4]	Jikai Dong, Bing Wang, Xinjie Wang, Chenxi Cao, Shikuan Chen, Wenli Du. Optimization of sensor deployment sequences for hazardous gas leakage monitoring and source term estimation[J]. 中国化学工程学报, 2023, 56(4): 169-179.
[5]	Shuangfei Zhao, Yingying Nie, Wenyan Zhang, Runze Hu, Lianzhu Sheng, Wei He, Ning Zhu, Yuguang Li, Dong Ji, Kai Guo. Microfluidic field strategy for enhancement and scale up of liquid–liquid homogeneous chemical processes by optimization of 3D spiral baffle structure[J]. 中国化学工程学报, 2023, 56(4): 255-265.
[6]	Xibao Zhang, Zhenghong Luo. Bubble size modeling approach for the simulation of bubble columns[J]. 中国化学工程学报, 2023, 53(1): 194-200.
[7]	Pan Zhang, Guanghui Chen, Weiwen Wang, Guodong Zhang, Huaming Wang. Analysis of the nutation and precession of the vortex core and the influence of operating parameters in a cyclone separator[J]. 中国化学工程学报, 2022, 46(6): 1-10.
[8]	Ye Zhang, Yong Gao, Peng Wang, Duo Na, Zhenming Yang, Jinsong Zhang. Solvent extraction with a three-dimensional reticulated hollow-strut SiC foam microchannel reactor[J]. 中国化学工程学报, 2022, 46(6): 53-62.
[9]	Mehdi Miansari, Mehdi Rajabtabar Darvishi, Davood Toghraie, Pouya Barnoon, Mojtaba Shirzad, As'ad Alizadeh. Numerical investigation of grooves effects on the thermal performance of helically grooved shell and coil tube heat exchanger[J]. 中国化学工程学报, 2022, 44(4): 424-434.
[10]	Shuai Chen, Jiahong Lan, Yu Zhang, Jia Guo, Zhikai Cao, Yong Sha. 3D multiphase flow simulation of Marangoni convection on reactive absorption of CO₂ by monoethanolamine in microchannel[J]. 中国化学工程学报, 2022, 43(3): 370-377.
[11]	Jian Chen, Lingbing Bu, Yingqi Luo. Comparative study on pressure swing adsorption system for industrial hydrogen and fuel cell hydrogen[J]. 中国化学工程学报, 2022, 42(2): 112-119.
[12]	Jing Zhang, Zhongyi Ge, Wei Wang, Bin Gong, Yaxia Li, Jianhua Wu. The concave-wall jet characteristics in vertical cylinder separator with inlet baffle component[J]. 中国化学工程学报, 2022, 42(2): 178-189.
[13]	Liwang Wang, Erwen Chen, Liang Ma, Zhanghuang Yang, Zongzhe Li, Weihui Yang, Hualin Wang, Yulong Chang. Numerical simulation and experimental study of gas cyclone–liquid jet separator for fine particle separation[J]. 中国化学工程学报, 2022, 51(11): 43-52.
[14]	Jie Ju, Xianjian Duan, Bismark Sarkodie, Yanjie Hu, Hao Jiang, Chunzhong Li. Numerical simulation of flow field and residence time of nanoparticles in a 1000-ton industrial multi-jet combustion reactor[J]. 中国化学工程学报, 2022, 51(11): 86-99.
[15]	Longyun Zheng, Kai Guo, Hongwei Cai, Bo Zhang, Hui Liu, Chunjiang Liu. Investigation of mass transfer model of CO₂ absorption with Rayleigh convection using multi-relaxation time lattice Boltzmann method[J]. 中国化学工程学报, 2022, 50(10): 130-142.

Effects of Gas Temperature Fluctuation on the Soot Formation Reactions

Effects of Gas Temperature Fluctuation on the Soot Formation Reactions

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价