Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed

doi:10.1016/j.cjche.2019.03.012

中国化学工程学报 ›› 2019, Vol. 27 ›› Issue (7): 1666-1673.DOI: 10.1016/j.cjche.2019.03.012

• Biotechnology and Bioengineering • 上一篇下一篇

Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed

Yong Huang^1,2,3,4,5,6, Ningbo Wang², Qiaoxia Liu², Wusheng Wang², Xiaoxun Ma^1,3,4,5,6

1 School of Chemical Engineering, Northwest University, 229 North Taibai Road, Xi'an 710069, China;
2 Hydrocarbon High-efficiency Utilization Technology Research Center of Yanchang Petroleum(Group) Co. Ltd., Xi'an 710075, China;
3 Chemical Engineering Research Center of the Ministry of Education(MOE) for Advanced Use Technology of Shanbei Energy, Xi'an 710069, China;
4 Shaanxi Research Center of Engineering Technology for Clean Coal Conversion, Xi'an 710069, China;
5 Collaborative Innovation Center for Development of Energy and Chemical Industry in Northern Shaanxi, Xi'an 710069, China;
6 International Scientific and Technological Cooperation Base of the Ministry of Science and Technology(MOST) for Clean Utilization of Hydrocarbon Resources, Xi'an 710069, China

收稿日期:2018-10-08 出版日期:2019-07-28 发布日期:2019-10-14
通讯作者: Xiaoxun Ma

Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed

Yong Huang^1,2,3,4,5,6, Ningbo Wang², Qiaoxia Liu², Wusheng Wang², Xiaoxun Ma^1,3,4,5,6

1 School of Chemical Engineering, Northwest University, 229 North Taibai Road, Xi'an 710069, China;
2 Hydrocarbon High-efficiency Utilization Technology Research Center of Yanchang Petroleum(Group) Co. Ltd., Xi'an 710075, China;
3 Chemical Engineering Research Center of the Ministry of Education(MOE) for Advanced Use Technology of Shanbei Energy, Xi'an 710069, China;
4 Shaanxi Research Center of Engineering Technology for Clean Coal Conversion, Xi'an 710069, China;
5 Collaborative Innovation Center for Development of Energy and Chemical Industry in Northern Shaanxi, Xi'an 710069, China;
6 International Scientific and Technological Cooperation Base of the Ministry of Science and Technology(MOST) for Clean Utilization of Hydrocarbon Resources, Xi'an 710069, China

Received:2018-10-08 Online:2019-07-28 Published:2019-10-14
Contact: Xiaoxun Ma

摘要/Abstract

摘要： An experimental study on co-pyrolysis of bituminous coal and biomass was performed in a pressured fluidized bed reactor. The blend ratio of biomass in the mixture was varied between 0 and 100 wt%, and the temperature was over a range of 550-650℃ under 1.0 MPa pressure with different atmospheres. On the basis of the individual pyrolysis behavior of bituminous coal and biomass, the influences of the biomass blending ratio, temperature, pressure and atmosphere on the product distribution were investigated. The results indicated that there existed a synergetic effect in the co-pyrolysis of bituminous coal and biomass in this pressured fluidized bed reactor, especially when the condition of bituminous coal and biomass blend ratio of 70:30 (w/w), 600℃, and 0.3 MPa was applied. The addition of biomass influenced the tar and char yields and gas and tar composition during co-pyrolysis. The tar yields were higher than the calculated values from individual pyrolysis of each fuel, and consequently the char yields were lower. The experimental results showed that the composition of the gaseous products was not in accordance with those of their individual fuel. The improvement of composition in tar also indicated synergistic effect in the co-pyrolysis.

关键词: Bituminous coal, Biomass, Co-pyrolysis, Pressured fluidized bed, Synergistic effect

Abstract: An experimental study on co-pyrolysis of bituminous coal and biomass was performed in a pressured fluidized bed reactor. The blend ratio of biomass in the mixture was varied between 0 and 100 wt%, and the temperature was over a range of 550-650℃ under 1.0 MPa pressure with different atmospheres. On the basis of the individual pyrolysis behavior of bituminous coal and biomass, the influences of the biomass blending ratio, temperature, pressure and atmosphere on the product distribution were investigated. The results indicated that there existed a synergetic effect in the co-pyrolysis of bituminous coal and biomass in this pressured fluidized bed reactor, especially when the condition of bituminous coal and biomass blend ratio of 70:30 (w/w), 600℃, and 0.3 MPa was applied. The addition of biomass influenced the tar and char yields and gas and tar composition during co-pyrolysis. The tar yields were higher than the calculated values from individual pyrolysis of each fuel, and consequently the char yields were lower. The experimental results showed that the composition of the gaseous products was not in accordance with those of their individual fuel. The improvement of composition in tar also indicated synergistic effect in the co-pyrolysis.

Key words: Bituminous coal, Biomass, Co-pyrolysis, Pressured fluidized bed, Synergistic effect

Yong Huang, Ningbo Wang, Qiaoxia Liu, Wusheng Wang, Xiaoxun Ma. Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed[J]. 中国化学工程学报, 2019, 27(7): 1666-1673.

Yong Huang, Ningbo Wang, Qiaoxia Liu, Wusheng Wang, Xiaoxun Ma. Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed[J]. Chinese Journal of Chemical Engineering, 2019, 27(7): 1666-1673.

参考文献

[1] L. Laopaiboon, P. Laopaiboon, Ethanol production from sweet sorghum juice in repeated-batch fermentation by Saccharomyces cerevisiae immobilized on corncob, World J. Microbiol. Biotechnol. 28(2012) 559-566.
[2] T. Silalertruksa, S.H. Gheewala, Security of feedstock supply for future bioethanol production in Thailand, Energy Policy 38(2010) 7476-7486.
[3] A.S. Bennett, R.P. Anex, Production, transportation and milling costs of sweet sorghum as a feedstock for centrifuged bioethanol production in the upper Midwest, Bioresour. Technol. 100(2009) 1595-1607.
[4] P. Jaisil, P. Pakdee, T. Pothisoong, K. Lertprasert-rat, Production cost of sweet sorghum (Sorghum bicolor (L.) Moench) and syrup production for ethanol plant, in:J. Nat. Res. Counc. Thai. (Energy). Special issue for 50th anniversary of NRCT, 2009, pp. 148-156.
[5] J.M. Bvochora, J.S. Read, R. Zvauya, Application of very high gravity technology to the cofermentation of sweet stem sorghum juice and sorghum grain, Ind. Crop. Prod. 11(2000) 11-17.
[6] F.W. Bai, L.J. Chen, Z. Zhang, W.A. Anderson, M. Moo-Yang, Continuous ethanol production and evaluation of yeast cell lysis and viability loss under very high gravity medium conditions, J. Biotechnol. 110(2004) 287-293.
[7] L.V.A. Reddy, O.V.S. Reddy, Rapid and enhanced production of ethanol in very high gravity (VHG) sugar fermentations by Saccharomyces cerevisiae:Role of finger millet (Eleusine coracana L.) flour, Process Biochem. 41(2006) 726-729.
[8] P. Chan-U-Tit, L. Laopaiboon, P. Jaisil, P. Laopaiboon, High level ethanol production by nitrogen and osmoprotectant supplementation under very high gravity fermentation conditions, Energies 6(2013) 884-899.
[9] L. Laopaiboon, S. Nuanpeng, P. Srinophakun, P. Klanrit, P. Laopaiboon, Ethanol production from sweet sorghum juice using very high gravity technology:Effects of carbon and nitrogen supplementations, Bioresour. Technol. 100(2009) 4176-4182.
[10] N. Khongsay, L. Laopaiboon, P. Jaisil, P. Laopaiboon, Optimization of agitation and aeration for very high gravity ethanol fermentation from sweet sorghum juice by Saccharomyces cerevisiae using orthogonal array design, Energies 5(2012) 561-576.
[11] S. Anastassiadis, H.J. Rehm, Citric acid production from glucose by yeast Candida oleophila ATCC20177 under batch, continuous and repeated batch cultivation, Electron. J. Biotechnol. 9(2006) 26-39.
[12] P. Ariyajarearnwong, L. Laopaiboon, P. Jaisil, P. Laopaiboon, Repeated-batch ethanol fermentation from sweet sorghum juice by free cell of Saccharomyces cerevisiae NP01, Afr. J. Biotechnol. 10(2011) 13909-13918.
[13] P.K. Herman, Stationary phase in yeast, Curr. Opin. Microbiol. 5(2002) 602-607.
[14] J.V. Gray, G.A. Petsko, G.C. Johnston, D. Ringe, R.A. Singer, M. WernerWashburne, ‘Sleeping beauty’:Quiescence in Saccharomyces cerevisiae, Microbiol. Mol. Biol. Rev. 68(2004) 187-206.
[15] I. Mannazzu, D. Angelozzi, S. Belviso, M. Budroni, G.A. Farris, P. Goffrini, T. Lodi, M. Marzona, L. Bardi, Behaviour of Saccharomyces cerevisiae wine strains during adaptation to unfavourable conditions of fermentation on synthetic medium:Cell lipid composition, membrane integrity, viability and fermentative activity, Int. J. Food Microbiol. 121(2008) 84-91.
[16] O. Deesuth, P. Laopaiboon, L. Laopaiboon, High ethanol production under optimal aeration conditions and yeast composition in a very high gravity fermentation from sweet sorghum juice by Saccharomyces cerevisiae, Ind. Crop. Prod. 92(2016) 263-270.
[17] M. Mecozzi, Estimation of total carbohydrate amount in environmental samples by the phenol sulphuric acid method assisted by multivariate calibration, Chemom. Intell. Lab. Syst. 79(2005) 84-90.
[18] B.W. Zoecklien, K.C. Fugelsang, B.H. Gump, F.S. Nury, Wine Analysis and Production, Chapman & Hall, New York, 1995.
[19] Association of Official Analytical Chemists (AOAC), Compendium of Methods for Food Analysis, 1997, pp. 2-18.
[20] T. Inoue, H. Iefuji, T. Fujii, H. Soga, K. Satoh, Cloning and characterization of a gene complementing the mutation of an ethanol-sensitive mutant of Sake yeast, Biosci. Biotechnol. Biochem. 64(2000) 229-236.
[21] J.P. Chen, K.W. Wu, H. Fukuda, Bioethanol production from uncooked raw starch by immobilized surface-engineered yeast cells, Appl. Biochem. Biotechnol. 67(2008) 59-67.
[22] S.N.R. Thammasittirong, T. Thirasaktana, A. Thammasittirong, M. Srisodsuk, Improvement of ethanol production by ethanol-tolerant Saccharomyces cerevisiae UVNR56, Springerplus 2(2013) 583-587.
[23] S. Nuangpeng, L. Laopaiboon, P. Srinophakun, P. Klanrit, P. Jaisil, P. Laopaiboon, Ethanol production from sweet sorghum juice under very high gravity conditions:Batch, repeated-batch and scale up for fermentation, Electron. J. Biotechnol. 14(2011) 1-12.
[24] S.H.M. Azhar, R. Abdulla, S.A. Jambo, H. Marbawi, J.A. Gansau, A.A.M. Faik, K.F. Rodrigues, Yeast in sustainable bioethanol production:A review, Biochem. Biophys. Rep. 10(2017) 52-61.
[25] M. Arshad, T. Hussain, M. Iqbal, M. Abbas, Enhanced ethanol production at commercial from molasses using high gravity technology by mutant S. cerevisiae, Braz. J. Microbiol. 48(2017) 403-409.
[26] G.Z. Breisha, Production of 16% ethanol from 35% sucrose, Biomass Bioenergy 34(2010) 1243-1249.
[27] Nurhayati Jayus, A. Mayzuhroh, S. Arindhani, C. Caroenchai, Studies on bioethanol production of commercial baker's and alcohol yeast under aerated culture using sugarcane molasses as the media, Agric. Agric. Sci. Procedia 9(2016) 493-499.
[28] F.W. Bai, X.Q. Zhao, High gravity ethanol fermentations and yeast tolerance, Microbiol. Monogr. 22(2012) 117-135.
[29] M. Siderius, O. van Wuytswinkel, K.A. Reijenga, M. Kelders, W.H. Mager, The control of intracellular glycerol in Saccharomyces cerevisiae influences osmotic stress response and resistance to increased temperature, Mol. Microbiol. 36(2000) 1381-1390.
[30] T. Modig, K. Granath, L. Adler, G. Liden, Anaerobic glycerol production by Saccharomyces cerevisiae strains under hyperosmotic stress, Appl. Microbiol. Biotechnol. 75(2007) 289-296.
[31] S. Alfenore, X. Cemeleyre, L. Benbadis, C. Bideaux, J.L. Uribelarrea, G. Goma, C. Molina-Jouve, S.E. Guillouet, Aeration strategy:A need for very high ethanol performance in Saccharomyces cerevisiae fed-batch process, Appl. Microbiol. Biotechnol. 63(2004) 537-542.
[32] O. Deesuth, P. Laopaiboon, P. Klanrit, L. Laopaiboon, Improvement of ethanol production from sweet sorghum juice under high gravity and very high gravity conditions:Effect of nutrient supplementation and aeration, Ind. Crop. Prod. 74(2015) 95-102.
[33] W.M. Ingledew, Alcohol production by Saccharomyces cerevisiae:A yeast primer, in:The Alcohol Textbook, 3rd ed., Nottingham University Press, UK, 1999.
[34] N. Khongsay, Y.H. Lin, P. Laopaiboon, L. Laopaiboon, Improvement of veryhigh-gravity ethanol fermentation from sweet sorghum juice by controlling fermentation redox potential, J. Taiwan Inst. Chem. Eng. 45(2014) 302-307.
[35] G. Zara, D. Angelozzi, S. Belviso, L. Bardi, P. Goffrini, T. Lodi, M. Budroni, I. Mannazzu, Oxygen is required to restore flor strain viability and lipid biosynthesis under fermentative conditions, FEMS Yeast Res. 9(2009) 217-225.
[36] W.P. Piper, The heat shock and ethanol stress response of yeast exhibit extensive similarity and functional overlap, FEMS Microbiol. Lett. 134(1995) 121-127.
[37] P. Mishra, S. Kaur, Lipids as modulators of ethanol tolerance in yeast, Appl. Microbiol. Biotechnol. 34(1991) 697-702.
[38] H. Alexandre, I. Rousseaux, C. Charpentier, Relationship between ethanol tolerance, lipid composition and plasma membrane fluidity in Saccharomyces cerevisiae and Kloeckera apiculata, FEMS Microbiol. Lett. 124(1994) 17-22.
[39] G. Beltran, M. Novo, J.M. Guillamón, A. Mas, N. Rozès, Effect of fermentation temperature and culture media on the yeast lipid composition and wine volatile compounds, Int. J. Food Microbiol. 121(2008) 169-177.
[40] F. Aguilera, R.A. Peinado, C. Millán, J.M. Ortega, J.C. Mauricio, Relationship between ethanol tolerance, H⁺-ATPase activity and the lipid composition of the plasma membrane in different wine yeast strains, Int. J. Food Microbiol. 110(2006) 34-42.
[41] F.W. Bai, W.A. Anderson, M. Moo-Young, Ethanol fermentation technologies from sugar and starch feedstocks, Biotechnol. Adv. 26(2008) 89-105.
[42] Y.H. Lin, W.S. Chien, K.J. Duan, P.R. Chang, Effect of aeration timing and interval during very-high-gravity ethanol fermentation, Process Biochem. 46(2011) 1025-1028.
[43] F.B. Pereira, P.M.R. Guimaraes, J.A. Teixeira, Robust industrial Saccharomyces cerevisiae strains for very high gravity bio-ethanol fermentations, J. Biosci. Bioeng. 112(2011) 130-136.

Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed

Co-pyrolysis of bituminous coal and biomass in a pressured fluidized bed

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价

[1]	Jian Han, Xinhua Liu, Shanwei Hu, Nan Zhang, Jingjing Wang, Bin Liang. Optimization of decoupling combustion characteristics of coal briquettes and biomass pellets in household stoves[J]. 中国化学工程学报, 2023, 59(7): 182-192.
[2]	Wei Wang, Romain Lemaire, Ammar Bensakhria, Denis Luart. Thermogravimetric analysis and kinetic modeling of the co-pyrolysis of a bituminous coal and poplar wood[J]. 中国化学工程学报, 2023, 58(6): 53-68.
[3]	Wende Tian, Jiawei Zhang, Zhe Cui, Haoran Zhang, Bin Liu. Microscopic mechanism study and process optimization of dimethyl carbonate production coupled biomass chemical looping gasification system[J]. 中国化学工程学报, 2023, 58(6): 291-305.
[4]	Qi Yang, Weikang Dai, Maoshuai Li, Jie Wei, Yi Feng, Cheng Yang, Wanxin Yang, Ying Zheng, Jie Ding, Mei-Yan Wang, Xinbin Ma. Enhanced selective hydrogenation of glycolaldehyde to ethylene glycol over Cu⁰-Cu⁺ sites[J]. 中国化学工程学报, 2023, 57(5): 141-150.
[5]	Mustapha Omenesa Idris, Claudia Guerrero-Barajas, Hyun-Chul Kim, Asim Ali Yaqoob, Mohamad Nasir Mohamad Ibrahim. Scalability of biomass-derived graphene derivative materials as viable anode electrode for a commercialized microbial fuel cell: A systematic review[J]. 中国化学工程学报, 2023, 55(3): 277-292.
[6]	Shutong Pang, Hualiang An, Xinqiang Zhao, Yanji Wang. Influence of Ca/P ratio on the catalytic performance of hydroxyapatite for decarboxylation of itaconic acid to methacrylic acid[J]. 中国化学工程学报, 2023, 53(1): 402-408.
[7]	Xing Zhang, Jingfeng Wu, Junhao Chen, Liang Lu, Lingjun Zhu, Shurong Wang. Production of aromatic hydrocarbons by co-cracking of bio-oil and ethanol over Ga₂O₃/HZSM-5 catalysts[J]. 中国化学工程学报, 2022, 46(6): 126-133.
[8]	Xiangjun Li, Shujun Li, Xiaoping Wang, Muhammad Asif Nawaz, Dianhua Liu. Polyoxymethylene dimethyl ethers synthesis from methanol and formaldehyde solution over one-pot synthesized spherical mesoporous sulfated zirconia[J]. 中国化学工程学报, 2022, 46(6): 161-172.
[9]	Zheng Wang, Sijia Li, Shengping Wang, Jiaxu Liu, Yujun Zhao, Xinbin Ma. Coupling effect of bifunctional ZnCe@SBA-15 catalyst in 1,3-butadiene production from bioethanol[J]. 中国化学工程学报, 2022, 45(5): 162-170.
[10]	Yanan Wei, Yunlei Zhang, Bing Li, Wen Guan, Changhao Yan, Xin Li, Yongsheng Yan. Facile synthesis of metal-organic frameworks embedded in interconnected macroporous polymer as a dual acid-base bifunctional catalyst for efficient conversion of cellulose to 5-hydroxymethylfurfural[J]. 中国化学工程学报, 2022, 44(4): 169-181.
[11]	Xuanyi Jia, Xiaomin Hu, Qiao Wang, Baiquan Chen, Xingyue Xie, Lihong Huang. Auto-thermal reforming of acetic acid for hydrogen production by Zn_xNi_yCrO_m±δ catalysts: Effect of Cr promoted Ni-Zn intermetallic compound[J]. 中国化学工程学报, 2022, 43(3): 216-221.
[12]	Wanyuan Wang, Chengxin Wen, Daoyuan Zheng, Chunhu Li, Junjie Bian, Xinbo Wang. Simultaneous degradation of RhB and reduction of Cr(VI) by MIL-53(Fe)/Polyaniline (PANI) with the mediation of organic acid[J]. 中国化学工程学报, 2022, 42(2): 55-63.
[13]	Peter Keliona Wani Likun, Huiyan Zhang, Yuyang Fan. Improving hydrocarbons production via catalytic co-pyrolysis of torrefied-biomass with plastics and dual catalytic pyrolysis[J]. 中国化学工程学报, 2022, 42(2): 196-209.
[14]	Kaili Zhang, Ligang Wei, Qingqin Sun, Jian Sun, Kunlan Li, Shangru Zhai, Qingda An, Junwang Zhang. Effects of formaldehyde on fermentable sugars production in the low-cost pretreatment of corn stalk based on ionic liquids[J]. 中国化学工程学报, 2022, 42(2): 406-414.
[15]	Yan Zhang, Jiaguang Zheng, Zhiyu Lu, Mengchen Song, Jiahuan He, Fuying Wu, Liuting Zhang. Boosting the hydrogen storage performance of magnesium hydride with metal organic framework-derived Cobalt@Nickel oxide bimetallic catalyst[J]. 中国化学工程学报, 2022, 52(12): 161-171.