Fundamental mechanisms and phenomena of clathrate hydrate nucleation

doi:10.1016/j.cjche.2018.12.016

中国化学工程学报 ›› 2019, Vol. 27 ›› Issue (9): 2014-2025.DOI: 10.1016/j.cjche.2018.12.016

• Special Issue on Natural Gas Hydrate • 上一篇下一篇

Fundamental mechanisms and phenomena of clathrate hydrate nucleation

Jinlong Cui¹, Zhenfeng Sun¹, Xiaohui Wang¹, Bin Yu², Shudong Leng², Guangjin Chen¹, Changyu Sun¹

1 State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China;
2 China Ship Design & Research Center Co., Ltd., Dalian 116001, China

收稿日期:2018-09-19 修回日期:2018-11-08 出版日期:2019-09-28 发布日期:2019-12-04
通讯作者: Xiaohui Wang, Changyu Sun
基金资助:
Supported by the National Key Research and Development Program of China (2016YFC0304003, 2017YFC0307302), the National Natural Science Foundation of China (21636009, 51576209, 21522609), and the Innovative Talents Support Program for Postgraduates (BX201700288).

Fundamental mechanisms and phenomena of clathrate hydrate nucleation

Jinlong Cui¹, Zhenfeng Sun¹, Xiaohui Wang¹, Bin Yu², Shudong Leng², Guangjin Chen¹, Changyu Sun¹

1 State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China;
2 China Ship Design & Research Center Co., Ltd., Dalian 116001, China

Received:2018-09-19 Revised:2018-11-08 Online:2019-09-28 Published:2019-12-04
Contact: Xiaohui Wang, Changyu Sun
Supported by:
Supported by the National Key Research and Development Program of China (2016YFC0304003, 2017YFC0307302), the National Natural Science Foundation of China (21636009, 51576209, 21522609), and the Innovative Talents Support Program for Postgraduates (BX201700288).

摘要/Abstract

摘要： Insights into the mechanism of hydrate nucleation are of great significance for the development of hydrate-based technologies, hydrate relevant flow assurance, and the exploration of in situ natural gas hydrates. Compared with the thermodynamics of hydrate formation, understanding the nucleation mechanism is challenging and has drawn substantial attention in recent decades. In this paper, we attempt to give a comprehensive review of the recent progress of studies of clathrate hydrate nucleation. First, the existing hypotheses on the hydrate nucleation mechanism are introduced and discussed. Then, we summarize recent experimental studies on induction time, a key parameter evaluating the velocity of the nucleation process. Subsequently, the memory effect is particularly discussed, followed by the suggestion of several promising research perspectives.

关键词: Hydrate, Nucleation, Mechanism, Induction time, Memory effect

Abstract: Insights into the mechanism of hydrate nucleation are of great significance for the development of hydrate-based technologies, hydrate relevant flow assurance, and the exploration of in situ natural gas hydrates. Compared with the thermodynamics of hydrate formation, understanding the nucleation mechanism is challenging and has drawn substantial attention in recent decades. In this paper, we attempt to give a comprehensive review of the recent progress of studies of clathrate hydrate nucleation. First, the existing hypotheses on the hydrate nucleation mechanism are introduced and discussed. Then, we summarize recent experimental studies on induction time, a key parameter evaluating the velocity of the nucleation process. Subsequently, the memory effect is particularly discussed, followed by the suggestion of several promising research perspectives.

Key words: Hydrate, Nucleation, Mechanism, Induction time, Memory effect

Jinlong Cui, Zhenfeng Sun, Xiaohui Wang, Bin Yu, Shudong Leng, Guangjin Chen, Changyu Sun. Fundamental mechanisms and phenomena of clathrate hydrate nucleation[J]. 中国化学工程学报, 2019, 27(9): 2014-2025.

Jinlong Cui, Zhenfeng Sun, Xiaohui Wang, Bin Yu, Shudong Leng, Guangjin Chen, Changyu Sun. Fundamental mechanisms and phenomena of clathrate hydrate nucleation[J]. Chinese Journal of Chemical Engineering, 2019, 27(9): 2014-2025.

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Fundamental mechanisms and phenomena of clathrate hydrate nucleation

Fundamental mechanisms and phenomena of clathrate hydrate nucleation

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