Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation

doi:10.1016/j.cjche.2021.03.014

中国化学工程学报 ›› 2022, Vol. 45 ›› Issue (5): 229-237.DOI: 10.1016/j.cjche.2021.03.014

Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation

Shenglin Yan¹, Yan Zhang¹, Chong Peng², Xiaoyong Yang¹, Yuan Huang³, Zhishan Bai¹, Xiao Xu¹

1 State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Mechanical and Power Engineering, East China University of Science and Technology, Shanghai 200237, China;
2 Sinopec Dalian Research Institute of Petroleum and Petrochemicals, Dalian 116041, China;
3 Institute of Environmental Pollution and Health, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China

收稿日期:2021-01-11 修回日期:2021-03-21 出版日期:2022-05-28 发布日期:2022-06-22
通讯作者: Zhishan Bai,E-mail:baizs@ecust.edu.cn
基金资助:
This research was supported by the National Natural Science Foundation of China (51578239) and the Education and Scientific Research Projects of Shanghai (17DZ1202802), for which the authors express their appreciation.

Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation

Shenglin Yan¹, Yan Zhang¹, Chong Peng², Xiaoyong Yang¹, Yuan Huang³, Zhishan Bai¹, Xiao Xu¹

1 State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Mechanical and Power Engineering, East China University of Science and Technology, Shanghai 200237, China;
2 Sinopec Dalian Research Institute of Petroleum and Petrochemicals, Dalian 116041, China;
3 Institute of Environmental Pollution and Health, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China

Received:2021-01-11 Revised:2021-03-21 Online:2022-05-28 Published:2022-06-22
Contact: Zhishan Bai,E-mail:baizs@ecust.edu.cn
Supported by:
This research was supported by the National Natural Science Foundation of China (51578239) and the Education and Scientific Research Projects of Shanghai (17DZ1202802), for which the authors express their appreciation.

摘要/Abstract

摘要： Flotation is an efficient pre-treatment technology for oily water. In this work, the interaction process between the moving oil droplet and the gas bubble was studied by high-speed camera and Bassset-Boussinesq-Oseen (BBO) theoretical model, and the experimental and simulation results of the oil droplet trajectory were compared. Moreover, the micro-particle image velocimetry system was utilized to observe the flow inside and outside of the moving oil droplet. The results show that the BBO model with the mobile bubble’s surface can reflect the velocity change trend of the oil droplet during the interaction process between the moving oil droplet and the gas bubble, but there are some significant differences between the experimental and simulation results. While the oil droplet is moving on the bubble’s surface, the velocity of the area near the contact point of oil droplet–gas bubble is less than that of the other areas inside the oil droplet. Meanwhile, the flow of water above the oil drop is more biased towards the gas bubble.

关键词: Flotation, Oil droplet–gas bubble interaction, Approach process, Hydrodynamics

Abstract: Flotation is an efficient pre-treatment technology for oily water. In this work, the interaction process between the moving oil droplet and the gas bubble was studied by high-speed camera and Bassset-Boussinesq-Oseen (BBO) theoretical model, and the experimental and simulation results of the oil droplet trajectory were compared. Moreover, the micro-particle image velocimetry system was utilized to observe the flow inside and outside of the moving oil droplet. The results show that the BBO model with the mobile bubble’s surface can reflect the velocity change trend of the oil droplet during the interaction process between the moving oil droplet and the gas bubble, but there are some significant differences between the experimental and simulation results. While the oil droplet is moving on the bubble’s surface, the velocity of the area near the contact point of oil droplet–gas bubble is less than that of the other areas inside the oil droplet. Meanwhile, the flow of water above the oil drop is more biased towards the gas bubble.

Key words: Flotation, Oil droplet–gas bubble interaction, Approach process, Hydrodynamics

Shenglin Yan, Yan Zhang, Chong Peng, Xiaoyong Yang, Yuan Huang, Zhishan Bai, Xiao Xu. Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation[J]. 中国化学工程学报, 2022, 45(5): 229-237.

参考文献

[1] B.H. Diya'uddeen, W.M.A.W. Daud, A.R. Abdul Aziz, Treatment technologies for petroleum refinery effluents:A review, Process. Saf. Environ. Prot. 89 (2) (2011) 95-105
[2] G.J. Rincón, E.J. la Motta, Simultaneous removal of oil and grease, and heavy metals from artificial bilge water using electro-coagulation/flotation, J. Environ. Manage. 144 (2014) 42-50
[3] E.T. Igunnu, G.Z. Chen, Produced water treatment technologies, Int. J. Low-Carbon Technol. 9 (3) (2014) 157-177
[4] OSPAR Commission, OSPAR Recommendation 2006/4 Amending OSPAR Recommendation 2001/1 for the Management of Produced Water from Offshore Installations, https://www.ospar.org/documents?d=32608., 2006.
[5] A.S. Heeres, J.J. Heijnen, L.A.M. van der Wielen, M.C. Cuellar, Gas bubble induced oil recovery from emulsions stabilised by yeast components, Chem. Eng. Sci. 145 (2016) 31-44
[6] H. Chakibi, I. Hénaut, A. Salonen, D. Langevin, J.F. Argillier, Role of bubble-drop interactions and salt addition in flotation performance, Energy Fuels 32 (3) (2018) 4049-4056
[7] M. Dudek, G. Øye, Microfluidic study on the attachment of crude oil droplets to gas bubbles, Energy Fuels 32 (10) (2018) 10513-10521
[8] R. Moosai, R.A. Dawe, Gas attachment of oil droplets for gas flotation for oily wastewater cleanup, Sep. Purif. Technol. 33 (3) (2003) 303-314
[9] S.L. Yan, X.Y. Yang, Z.S. Bai, X. Xu, H.L. Wang, Drop attachment behavior of oil droplet-gas bubble interactions during flotation, Chem. Eng. Sci. 223 (2020) 115740
[10] W.T. Strickland Jr, Laboratory results of cleaning produced water by gas flotation, Soc. Petroleum Eng. J. 20 (3) (1980) 175-190
[11] M. Eftekhardadkhah, S.V. Aanesen, K. Rabe, G. Øye, Oil removal from produced water during laboratory- and pilot-scale gas flotation:the influence of interfacial adsorption and induction times, Energy Fuels 29 (11) (2015) 7734-7740
[12] M. Eftekhardadkhah, G. Oye, Induction and coverage times for crude oil droplets spreading on air bubbles, Environ. Sci. Technol. 47 (24) (2013) 14154-14160
[13] I. Sven-Nilsson, Einfluß der Berührungszeitzwischen Mineral und Luftblase Bei der Flotation, Kolloid-Zeitschrift 69 (2) (1934) 230-232
[14] D.I. Verrelli, P.T.L. Koh, A.V. Nguyen, Particle-bubble interaction and attachment in flotation, Chem. Eng. Sci. 66 (23) (2011) 5910-5921
[15] A.V. Nguyen, A.H.J. Schulze, Colloidal Science of Flotation, Marcel Dekker, New York, 2004
[16] A.V. Nguyen, D.A. An-Vo, T. Tran-Cong, G.M. Evans, A review of stochastic description of the turbulence effect on bubble-particle interactions in flotation, Int. J. Miner. Process. 156 (2016) 75-86
[17] S. Goel, G.J. Jameson, Detachment of particles from bubbles in an agitated vessel, Miner. Eng. 36-38 (2012) 324-330
[18] T.Y. Liu, M.P. Schwarz, CFD-based multiscale modelling of bubble-particle collision efficiency in a turbulent flotation cell, Chem. Eng. Sci. 64 (24) (2009) 5287-5301
[19] J.B. Yianatos, Fluid flow and kinetic modelling in flotation related processes, Chem. Eng. Res. Des. 85 (12) (2007) 1591-1603
[20] H. Darabi, S.M.J. Koleini, D. Deglon, B. Rezai, M. Abdollahy, Particle image velocimetry study of the turbulence characteristics in an aerated flotation cell, Ind. Eng. Chem. Res. 56 (46) (2017) 13919-13928
[21] H. Schubert, C. Bischofberger, On the microprocesses air dispersion and particle-bubble attachment in flotation machines as well as consequences for the scale-up of macroprocesses, Int. J. Miner. Process. 52 (4) (1998) 245-259
[22] C.M. Phan, A.V. Nguyen, J.D. Miller, G.M. Evans, G.J. Jameson, Investigations of bubble-particle interactions, Int. J. Miner. Process. 72 (1-4) (2003) 239-254
[23] V. Sarrot, P. Guiraud, D. Legendre, Determination of the collision frequency between bubbles and particles in flotation, Chem. Eng. Sci. 60 (22) (2005) 6107-6117
[24] A.V. Nguyen, L. Alexandrova, L. Grigorov, G.J. Jameson, Dewetting kinetics on silica substrates:Three phase contact expansion measurements for aqueous dodecylammonium chloride films, Miner. Eng. 19 (6-8) (2006) 651-658
[25] B. Shahbazi, B. Rezai, S.M. JavadKoleini, Bubble-particle collision and attachment probability on fine particles flotation, Chem. Eng. Process.:Process. Intensif. 49 (6) (2010) 622-627
[26] Z. Brabcová, T. Karapantsios, M. Kostoglou, P. Basařová, K. Matis, Bubble-particle collision interaction in flotation systems, Colloids Surfaces A:Physicochem. Eng. Aspects 473 (2015) 95-103
[27] M. Firouzi, A.V. Nguyen, S.H. Hashemabadi, The effect of microhydrodynamics on bubble-particle collision interaction, Miner. Eng. 24 (9) (2011) 973-986
[28] W. Thielicke, E.J. Stamhuis, PIVlab-towards user-friendly, affordable and accurate digital particle image velocimetry in MATLAB, J. Open Res. Softw. 2 (2014) 30
[29] A.V. Nguyen, G.M. Evans, Movement of fine particles on an air bubble surface studied using high-speed video microscopy, J. Colloid Interface Sci. 273 (1) (2004) 271-277
[30] Z.L. Liu, Y. Zheng, PIV study of bubble rising behavior, Powder Technol. 168 (1) (2006) 10-20

Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation

Oil droplet movement and micro-flow characteristics during interaction process between gas bubble and oil droplet in flotation

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价

[1]	Tian Zhang, Qingshan Huang, Shujun Geng, Aqiang Chen, Yan Liu, Haidong Zhang. Impacts of solid physical properties on the performances of a slurry external airlift loop reactor integrating mixing and separation[J]. 中国化学工程学报, 2023, 55(3): 1-12.
[2]	Danlong Li, Yannan Liang, Hainan Wang, Ruoqian Zhou, Xiaokang Yan, Lijun Wang, Haijun Zhang. Investigation on the effects of fluid intensification based preconditioning process on the decarburization enhancement of fly ash[J]. 中国化学工程学报, 2022, 44(4): 275-283.
[3]	Wen-Cong Chen, Ya-Wei Fan, Liang-Liang Zhang, Bao-Chang Sun, Yong Luo, Hai-Kui Zou, Guang-Wen Chu, Jian-Feng Chen. Computational fluid dynamic simulation of gas-liquid flow in rotating packed bed: A review[J]. 中国化学工程学报, 2022, 41(1): 85-108.
[4]	Le Li, Yansheng Zhao, Wenhao Lian, Chun Han, Qian Zhang, Wei Huang. Review on the effect of heat exchanger tubes on flow behavior and heat/mass transfer of the bubble/slurry reactors[J]. 中国化学工程学报, 2021, 35(7): 44-61.
[5]	Yangjun Wei, Leming Cheng, Erdong Wu, Liyao Li. Experimental research on steady-state operation characteristics of gas-solid flow in a 15.5 m dual circulating fluidized bed system[J]. 中国化学工程学报, 2021, 32(4): 70-76.
[6]	Shuo Yang, Jilong Zhang, Jiaxing Xue, Qingpeng Wu, Qunsheng Li, Hongkang Zhao, Liqun Zhang. Hydrodynamics and mass transfer performance analysis of flow-guided trapezoid spray packing tray[J]. 中国化学工程学报, 2021, 39(11): 59-67.
[7]	Hongyan Liu, Zhuo Li, Shujun Geng, Fei Gao, Taobo He, Qingshan Huang. Influences of top clearance and liquid throughput on the performances of an external loop airlift slurry reactor integrated mixing and separation[J]. 中国化学工程学报, 2020, 28(6): 1514-1521.
[8]	Chenghui Zheng, Jiashun Guo, Chengkai Wang, Yuanfeng Chen, Huidong Zheng, Zuoyi Yan, Qinggen Chen. Experimental study and simulation of a three-phase flow stirred bioreactor[J]. 中国化学工程学报, 2019, 27(3): 649-659.
[9]	Kang Yu, Weijie Wang, Tao Zhang, Yumei Yong, Chao Yang. Effects of internals on phase holdup and backmixing in a slightlyexpanded-bed reactor with gas-liquid concurrent upflow[J]. 中国化学工程学报, 2019, 27(10): 2273-2283.
[10]	Yongzheng Li, Xiaolai Zhang, Guangwei Zhai, Haitao Zhang, Tao Li, Qiwen Sun, Weiyong Ying. LDV measurements of particle velocity distribution in an annular stripper[J]. 中国化学工程学报, 2019, 27(10): 2293-2303.
[11]	Xiaoli Wang, Lei Huang, Chunhua Yang. Prediction model of slurry pH based on mechanism and error compensation for mineral flotation process[J]. Chinese Journal of Chemical Engineering, 2018, 26(8): 1766-1772.
[12]	Dan Li, Kai Guo, Jingnan Li, Yiping Huang, Junchao Zhou, Hui Liu, Chunjiang Liu. Hydrodynamics and bubble behaviour in a three-phase two-stage internal loop airlift reactor[J]. Chinese Journal of Chemical Engineering, 2018, 26(6): 1359-1369.
[13]	Saad H. Ammar, Ahmed S. Akbar. Oilfield produced water treatment in internal-loop airlift reactor using electrocoagulation/flotation technique[J]. Chinese Journal of Chemical Engineering, 2018, 26(4): 879-885.
[14]	Zhineng Wang, Yong Kang, Xiaochuan Wang, Shijing Wu, Xiaoyong Li. Investigation of the hydrodynamics of slug flow in airlift pumps[J]. Chinese Journal of Chemical Engineering, 2018, 26(12): 2391-2402.
[15]	Hongkang Zhao, Lun Li, Baohua Wang, Dan Yu, Qunsheng Li. Hydrodynamics performance and tray efficiency analysis of the novel vertical spray packing tray[J]. Chinese Journal of Chemical Engineering, 2018, 26(12): 2448-2454.