SCI和EI收录∣中国化工学会会刊

›› 2017, Vol. 25 ›› Issue (3): 288-293.DOI: 10.1016/j.cjche.2016.08.021

• Separation Science and Engineering • 上一篇    下一篇

Prediction of mass transfer coefficients in an asymmetric rotating disk contactor using effective diffusivity

Meisam Torab-Mostaedi, Mehdi Asadollahzadeh, Jaber Safdari   

  1. Nuclear Fuel Cycle Research School, Nuclear Science and Technology Research Institute, P. O. Box:11365-8486, Tehran, Iran
  • 收稿日期:2016-05-31 修回日期:2016-08-23 出版日期:2017-03-28 发布日期:2017-04-15
  • 通讯作者: Mehdi Asadollahzadeh

Prediction of mass transfer coefficients in an asymmetric rotating disk contactor using effective diffusivity

Meisam Torab-Mostaedi, Mehdi Asadollahzadeh, Jaber Safdari   

  1. Nuclear Fuel Cycle Research School, Nuclear Science and Technology Research Institute, P. O. Box:11365-8486, Tehran, Iran
  • Received:2016-05-31 Revised:2016-08-23 Online:2017-03-28 Published:2017-04-15

摘要: Mass transfer characteristics have been investigated in a 113 mm diameter asymmetric rotating disk contactor of the pilot plant scale for two different liquid-liquid systems. The effects of operating parameters including rotor speed and continuous and dispersed phase velocities on the volumetric overall mass transfer coefficients are investigated. The results show that the mass transfer performance is strongly dependent on agitation rate and interfacial tension, but only slightly dependent on phase flow rates. In this study, effective diffusivity is used instead of molecular diffusivity in the Gröber equation for estimation of dispersed phase overall mass transfer coefficient. The enhancement factor is determined experimentally and there from an empirical expression is derived for prediction of the enhancement factor as a function of Reynolds number. The predicted results compared to the experimental data show that the proposed correlation can efficiently predict the overall mass transfer coefficients in asymmetric rotating disk contactors.

关键词: Asymmetric rotating disk contactor, Mass transfer coefficient, Enhancement factor, Interfacial area, Dispersed phase holdup

Abstract: Mass transfer characteristics have been investigated in a 113 mm diameter asymmetric rotating disk contactor of the pilot plant scale for two different liquid-liquid systems. The effects of operating parameters including rotor speed and continuous and dispersed phase velocities on the volumetric overall mass transfer coefficients are investigated. The results show that the mass transfer performance is strongly dependent on agitation rate and interfacial tension, but only slightly dependent on phase flow rates. In this study, effective diffusivity is used instead of molecular diffusivity in the Gröber equation for estimation of dispersed phase overall mass transfer coefficient. The enhancement factor is determined experimentally and there from an empirical expression is derived for prediction of the enhancement factor as a function of Reynolds number. The predicted results compared to the experimental data show that the proposed correlation can efficiently predict the overall mass transfer coefficients in asymmetric rotating disk contactors.

Key words: Asymmetric rotating disk contactor, Mass transfer coefficient, Enhancement factor, Interfacial area, Dispersed phase holdup