Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation

doi:10.1016/j.cjche.2019.03.029

中国化学工程学报 ›› 2019, Vol. 27 ›› Issue (10): 2560-2565.DOI: 10.1016/j.cjche.2019.03.029

• Energy, Resources and Environmental Technology • 上一篇下一篇

Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation

Li Peng¹, Limin Wang¹, Feng Zhu¹, Jinyun Liu¹, Wenfu Yan², Xuehong Gu¹

1 State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing 210009, China;
2 State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, China

收稿日期:2018-11-26 修回日期:2019-03-20 出版日期:2019-10-28 发布日期:2020-01-17
通讯作者: Xuehong Gu
基金资助:
Supported by the National Natural Science Foundation of China (21490585, 21606126, 21176117), National High-tech Research and Development Program of China (2015AA03A602), the Outstanding Young Fund of Jiangsu Province (BK2012040), the "Six Top Talents" and "333 Talent Project" of Jiangsu Province, State Key Laboratory of Materials-Oriented Chemical Engineering (ZK201719) and the State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University (2018-19).

Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation

Li Peng¹, Limin Wang¹, Feng Zhu¹, Jinyun Liu¹, Wenfu Yan², Xuehong Gu¹

1 State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing 210009, China;
2 State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Changchun 130012, China

Received:2018-11-26 Revised:2019-03-20 Online:2019-10-28 Published:2020-01-17
Contact: Xuehong Gu
Supported by:
Supported by the National Natural Science Foundation of China (21490585, 21606126, 21176117), National High-tech Research and Development Program of China (2015AA03A602), the Outstanding Young Fund of Jiangsu Province (BK2012040), the "Six Top Talents" and "333 Talent Project" of Jiangsu Province, State Key Laboratory of Materials-Oriented Chemical Engineering (ZK201719) and the State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University (2018-19).

摘要/Abstract

摘要： A hollow-fiber-supported stable Au/FAU catalytic membrane was successfully synthesized through a polydopamine coating modification-removal strategy and used as a flow-through catalytic membrane reactor for preferential oxidation of CO. Small Au nanoparticles can be efficiently isolated by dopamine and the dopamine-derived carbon shells. The interactions between Au nanoparticles and zeolite layer support are enhanced during annealing at high temperature under an inert atmosphere. A zeolite membrane supported Au nanoparticle catalyst was obtained after the removal of carbon shells, which showed high catalytic activity and stability for the removal of CO from hydrogen.

关键词: Zeolite membrane, CO oxidation, Gold catalyst, Surface modification

Abstract: A hollow-fiber-supported stable Au/FAU catalytic membrane was successfully synthesized through a polydopamine coating modification-removal strategy and used as a flow-through catalytic membrane reactor for preferential oxidation of CO. Small Au nanoparticles can be efficiently isolated by dopamine and the dopamine-derived carbon shells. The interactions between Au nanoparticles and zeolite layer support are enhanced during annealing at high temperature under an inert atmosphere. A zeolite membrane supported Au nanoparticle catalyst was obtained after the removal of carbon shells, which showed high catalytic activity and stability for the removal of CO from hydrogen.

Key words: Zeolite membrane, CO oxidation, Gold catalyst, Surface modification

Li Peng, Limin Wang, Feng Zhu, Jinyun Liu, Wenfu Yan, Xuehong Gu. Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation[J]. 中国化学工程学报, 2019, 27(10): 2560-2565.

Li Peng, Limin Wang, Feng Zhu, Jinyun Liu, Wenfu Yan, Xuehong Gu. Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation[J]. Chinese Journal of Chemical Engineering, 2019, 27(10): 2560-2565.

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Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation

Polydopamine modified Au/FAU catalytic membrane for CO preferential oxidation

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